Integration of commercial screen-printed electrodes into a voltammetric electronic tongue for the analysis of aminothiols

A voltammetric sensor array (or electronic tongue) is developed for the simultaneous quantification of cysteine, glutathione and homocysteine without need of previous separation. It is based on the integration of three commercial screen-printed electrodes (gold curated at high and low temperature an...

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Detalles Bibliográficos
Autores: De Paula Pedroza, Ricardo Henrique, Serrano i Plana, Núria, Díaz Cruz, José Manuel, Ariño Blasco, Cristina, Esteban i Cortada, Miquel
Tipo de recurso: artículo
Estado:Versión aceptada para publicación
Fecha de publicación:2016
País:España
Institución:Universidad de Barcelona
Repositorio:Dipòsit Digital de la UB
OAI Identifier:oai:diposit.ub.edu:2445/140639
Acceso en línea:https://hdl.handle.net/2445/140639
Access Level:acceso abierto
Palabra clave:Voltametria
Cisteïna
Glutatió
Voltammetry
Cysteine
Glutathione
Descripción
Sumario:A voltammetric sensor array (or electronic tongue) is developed for the simultaneous quantification of cysteine, glutathione and homocysteine without need of previous separation. It is based on the integration of three commercial screen-printed electrodes (gold curated at high and low temperature and carbon modified with carbon nanotubes). Linear sweep voltammograms measured simultaneously by all three sensors are processed by Partial Least Squares (PLS) regression and different variables selection algorithms such as Genetic Algorithm and interval-Partial Least Squares. The method was applied to synthetic mixtures and successfully validated, with correlation coefficients of prediction (Rp2) of 0.9542, 0.9429 and 0.9589 for cysteine, glutathione, and homocysteine respectively.