Field-induced transitions and magnetization reserval in ErxY1-xCo0.50Mn0.50O3 (0.0 ≤ x ≤ 1.0)

[EN] Magnetic properties of the Er(Co,Mn)O3 solid solution result from a subtle interplay of different interactions between erbium moments and several other magnetic entities present in this system: Mn3+, Mn4+, Co2+, Co3+, as well as double-exchange interactions among them. The special case of the 0...

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Autores: Moure Jiménez, Carlos, Gil, Vanesa, Peña, Octavio, Allegret Maret, V., Antunes, A. B., Baibich, M. N.
Tipo de recurso: artículo
Fecha de publicación:2008
País:España
Institución:Consejo Superior de Investigaciones Científicas (CSIC)
Repositorio:DIGITAL.CSIC. Repositorio Institucional del CSIC
OAI Identifier:oai:digital.csic.es:10261/6448
Acceso en línea:http://hdl.handle.net/10261/6448
Access Level:acceso abierto
Palabra clave:Field-induced transitions
Spin reversal
Magnetic domains
Dynamical transitions
Transiciones inducidas por campo
Inversión de spin
Dominios magnéticos
Transiciones dinámicas
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spelling Field-induced transitions and magnetization reserval in ErxY1-xCo0.50Mn0.50O3 (0.0 ≤ x ≤ 1.0)Transiciones inducidas por campo e inversión de la imanación en ErxY1-xCo0.50Mn0.50O3 (0.0 ≤ x ≤ 1.0)Moure Jiménez, CarlosGil, VanesaPeña, OctavioAllegret Maret, V.Antunes, A. B.Baibich, M. N.Field-induced transitionsSpin reversalMagnetic domainsDynamical transitionsTransiciones inducidas por campoInversión de spinDominios magnéticosTransiciones dinámicas[EN] Magnetic properties of the Er(Co,Mn)O3 solid solution result from a subtle interplay of different interactions between erbium moments and several other magnetic entities present in this system: Mn3+, Mn4+, Co2+, Co3+, as well as double-exchange interactions among them. The special case of the 0.5:0.5 = Co:Mn substitution is particularly important since ferromagnetic domains may reorientate both under low and high external magnetic fields. Magnetic dilution of the erbium sublattice by non-magnetic yttrium (same valence and size) allows separating out the antiferromagnetic 4f-3d interactions leaving just the ferromagnetic Co2+-Mn4+ transition metal sublattice. Magnetic properties of the ErxY1-xCo0.50Mn0.50O3 (0.0 ≤ x ≤ 1.0) solid solution are presented, going from ferromagnetism (x = 0; YCo0.5Mn0.5O3) to ferrimagnetism (x = 1; ErCo0.5Mn0.5O3). Antiferromagnetic interactions get stronger while the Co/Mn ferromagnetic domains become harder to rotate when the rare-earth sublattice is progressively filled with erbium ions of large magnetic moments. A linear dependence with x(Er) is observed for the critical field Hcrit related to the reorientation of domains, going from 1.3 T up to 3.5 T, for x = 0 and 1, respectively. At the same time, the compensation temperature Tcomp increases and the spontaneous magnetization Mrem decreases with increasing content of erbium.[ES] Las propiedades magnéticas de las soluciones sólidas ErxY1-xCo0.50Mn0.50O3 (0.0 ≤ x ≤ 1.0) son consecuencia de una sutil interrelación de las diferentes interacciones entre los momentos magnéticos del Er3+ y de otras entidades magnéticas presentes en el sistema: Mn3+, Mn4+, Co2+, Co3+, así como las interacciones de doble canje entre ellas. El caso especial de la sustitución 0.5:0.5 = Co:Mn es particularmente importante puesto que los dominios ferromagnéticos pueden reorientarse bien con campos externos bajos como con altos. La dilución magnética de la subred de Er3+ por el ión no-magnético Y3+ (del mismo tamaño y valencia) permite separar las interacciones antiferromagnéticas 4f-3d dejando solamente las interacciones ferromagnéticas Co2+-Mn4+ de la subred de los metales de transición. Las propiedades magnéticas de las soluciones sólidas ErxY1-xCo0.50Mn0.50O3 (0.0 ≤ x ≤ 1.0) se presentan como variando desde ferromagnetismo (x = 0; YCo0.5Mn0.5O3) a ferrimagnetismo (x = 1; ErCo0.5Mn0.5O3). Las interacciones antiferromagnéticas se hacen más fuertes mientras que los dominios ferromagnéticos se hacen más difíciles de rotar cuando la subred de la tierra rara se va llenando progresivamente con iones Er3+, de momento magnético alto. Se observa una dependencia lineal con x(Er) del campo crítico Hcrit relacionado con la reorientación de dominios, variando desde 1.3 T hasta 3.5 T, para x = 0 y 1, respectivamente. Al mismo tiempo, la temperatura de compensación, Tcomp aumenta y la magnetización espontánea, Mrem disminuye con el contenido creciente de Er3+.Authors acknowledge the bilateral exchange programs France-Spain CNRS-CSIC, project n° 18873, and France-Brazil CAPES-COFECUB, project 416/03.Peer reviewedSociedad Española de Cerámica y Vidrio200820082008info:eu-repo/semantics/articlehttp://purl.org/coar/resource_type/c_6501423216 bytesapplication/pdfhttp://hdl.handle.net/10261/6448reponame:DIGITAL.CSIC. Repositorio Institucional del CSICinstname:Consejo Superior de Investigaciones Científicas (CSIC)Ingléshttp://boletines.secv.es/es/index.php?id=30&vol=47info:eu-repo/semantics/openAccessoai:digital.csic.es:10261/64482026-05-22T06:33:51Z
dc.title.none.fl_str_mv Field-induced transitions and magnetization reserval in ErxY1-xCo0.50Mn0.50O3 (0.0 ≤ x ≤ 1.0)
Transiciones inducidas por campo e inversión de la imanación en ErxY1-xCo0.50Mn0.50O3 (0.0 ≤ x ≤ 1.0)
title Field-induced transitions and magnetization reserval in ErxY1-xCo0.50Mn0.50O3 (0.0 ≤ x ≤ 1.0)
spellingShingle Field-induced transitions and magnetization reserval in ErxY1-xCo0.50Mn0.50O3 (0.0 ≤ x ≤ 1.0)
Moure Jiménez, Carlos
Field-induced transitions
Spin reversal
Magnetic domains
Dynamical transitions
Transiciones inducidas por campo
Inversión de spin
Dominios magnéticos
Transiciones dinámicas
title_short Field-induced transitions and magnetization reserval in ErxY1-xCo0.50Mn0.50O3 (0.0 ≤ x ≤ 1.0)
title_full Field-induced transitions and magnetization reserval in ErxY1-xCo0.50Mn0.50O3 (0.0 ≤ x ≤ 1.0)
title_fullStr Field-induced transitions and magnetization reserval in ErxY1-xCo0.50Mn0.50O3 (0.0 ≤ x ≤ 1.0)
title_full_unstemmed Field-induced transitions and magnetization reserval in ErxY1-xCo0.50Mn0.50O3 (0.0 ≤ x ≤ 1.0)
title_sort Field-induced transitions and magnetization reserval in ErxY1-xCo0.50Mn0.50O3 (0.0 ≤ x ≤ 1.0)
dc.creator.none.fl_str_mv Moure Jiménez, Carlos
Gil, Vanesa
Peña, Octavio
Allegret Maret, V.
Antunes, A. B.
Baibich, M. N.
author Moure Jiménez, Carlos
author_facet Moure Jiménez, Carlos
Gil, Vanesa
Peña, Octavio
Allegret Maret, V.
Antunes, A. B.
Baibich, M. N.
author_role author
author2 Gil, Vanesa
Peña, Octavio
Allegret Maret, V.
Antunes, A. B.
Baibich, M. N.
author2_role author
author
author
author
author
dc.subject.none.fl_str_mv Field-induced transitions
Spin reversal
Magnetic domains
Dynamical transitions
Transiciones inducidas por campo
Inversión de spin
Dominios magnéticos
Transiciones dinámicas
topic Field-induced transitions
Spin reversal
Magnetic domains
Dynamical transitions
Transiciones inducidas por campo
Inversión de spin
Dominios magnéticos
Transiciones dinámicas
description [EN] Magnetic properties of the Er(Co,Mn)O3 solid solution result from a subtle interplay of different interactions between erbium moments and several other magnetic entities present in this system: Mn3+, Mn4+, Co2+, Co3+, as well as double-exchange interactions among them. The special case of the 0.5:0.5 = Co:Mn substitution is particularly important since ferromagnetic domains may reorientate both under low and high external magnetic fields. Magnetic dilution of the erbium sublattice by non-magnetic yttrium (same valence and size) allows separating out the antiferromagnetic 4f-3d interactions leaving just the ferromagnetic Co2+-Mn4+ transition metal sublattice. Magnetic properties of the ErxY1-xCo0.50Mn0.50O3 (0.0 ≤ x ≤ 1.0) solid solution are presented, going from ferromagnetism (x = 0; YCo0.5Mn0.5O3) to ferrimagnetism (x = 1; ErCo0.5Mn0.5O3). Antiferromagnetic interactions get stronger while the Co/Mn ferromagnetic domains become harder to rotate when the rare-earth sublattice is progressively filled with erbium ions of large magnetic moments. A linear dependence with x(Er) is observed for the critical field Hcrit related to the reorientation of domains, going from 1.3 T up to 3.5 T, for x = 0 and 1, respectively. At the same time, the compensation temperature Tcomp increases and the spontaneous magnetization Mrem decreases with increasing content of erbium.
publishDate 2008
dc.date.none.fl_str_mv 2008
2008
2008
dc.type.none.fl_str_mv info:eu-repo/semantics/article
http://purl.org/coar/resource_type/c_6501
format article
dc.identifier.none.fl_str_mv http://hdl.handle.net/10261/6448
url http://hdl.handle.net/10261/6448
dc.language.none.fl_str_mv Inglés
language_invalid_str_mv Inglés
dc.relation.none.fl_str_mv http://boletines.secv.es/es/index.php?id=30&vol=47
dc.rights.none.fl_str_mv info:eu-repo/semantics/openAccess
eu_rights_str_mv openAccess
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dc.publisher.none.fl_str_mv Sociedad Española de Cerámica y Vidrio
publisher.none.fl_str_mv Sociedad Española de Cerámica y Vidrio
dc.source.none.fl_str_mv reponame:DIGITAL.CSIC. Repositorio Institucional del CSIC
instname:Consejo Superior de Investigaciones Científicas (CSIC)
instname_str Consejo Superior de Investigaciones Científicas (CSIC)
reponame_str DIGITAL.CSIC. Repositorio Institucional del CSIC
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