Determination of free and derivative terpenoids and sterols in spent coffee grounds by two-dimensional liquid chromatography coupled to high-resolution mass spectrometry

Spent coffee grounds (SCGs) are a major global waste, yet rich in valuable bioactive compounds. Unlocking their potential requires advanced analytical techniques due to the complexity of their molecular composition. This study presents an innovative RPLC × SFC-HRMS method—an online two-dimensional l...

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Detalles Bibliográficos
Autores: Caño-Carrillo, Irene, Batteau, Magali, Bruna, Lauriane, Gilbert-López, Bienvenida, García-Reyes, Juan F., Chatel, Gregory, Faure, Karine
Tipo de recurso: artículo
Estado:Versión aceptada para publicación
Fecha de publicación:2025
País:España
Institución:Universidad de Jaén
Repositorio:RUJA. Repositorio Institucional de la Producción Científica de la Universidad de Jaén
OAI Identifier:oai:ruja.ujaen.es:10953/6320
Acceso en línea:https://doi.org/10.1016/j.foodchem.2025.144853
https://hdl.handle.net/10953/6320
Access Level:acceso abierto
Palabra clave:Spent coffee grounds
liquid chromatography, supercritical fluid chromatography, online LCxSFC-HRMS
sterols
diterpenes
2301.03
2301.10
Descripción
Sumario:Spent coffee grounds (SCGs) are a major global waste, yet rich in valuable bioactive compounds. Unlocking their potential requires advanced analytical techniques due to the complexity of their molecular composition. This study presents an innovative RPLC × SFC-HRMS method—an online two-dimensional liquid chromatography approach—for simultaneous analysis of sterol and diterpene derivatives in SCGs. Using a custom-built interface, both free and esterified lipid fractions were analyzed directly from intact, non-saponified and non-derivatized extracts. The method effectively resolved isomeric compounds and sterol oxidation products, highlighting its power for comprehensive lipid profiling and paving the way for SCG valorization in health-focused applications.