Sequential trypsin and ProAlanase digestions unearth immunological protein biomarkers shrouded by skeletal collagen

This study investigates the efficacy of proteomic analysis of human remains to identify active infections in the past through the detection of pathogens and the host response to infection. We advance leprosy as a case study due to the sequestering of sufferers in leprosaria and the suggestive skelet...

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Detalles Bibliográficos
Autores: Wilkin, Shevan, Lanigan, Liam T., Montes, Nuria, Sharma, Mukul, Avanzi, Charlotte|||0000-0002-1062-4058, Sejdiu, Donikë, Majander, Kerttu|||0000-0002-7922-4482, Pfrengle, Saskia, Chiang, Yun, Kunz, Laura, Dittmann, Antje|||0000-0002-2570-5192, Rühli, Frank, Singh, Pushpendra, Coll, Maria Fontanals, Collins, Matthew J., Taurozzi, Alberto J., Schuenemann, Verena J.|||0000-0002-8593-3672
Tipo de recurso: artículo
Fecha de publicación:2024
País:España
Institución:Universitat Autònoma de Barcelona
Repositorio:Dipòsit Digital de Documents de la UAB
Idioma:inglés
OAI Identifier:oai:ddd.uab.cat:310541
Acceso en línea:https://ddd.uab.cat/record/310541
https://dx.doi.org/urn:doi:10.1016/j.isci.2024.109663
Access Level:acceso abierto
Palabra clave:Biochemistry
Biochemistry applications
Biochemistry methods
Medical biochemistry
Proteomics
Descripción
Sumario:This study investigates the efficacy of proteomic analysis of human remains to identify active infections in the past through the detection of pathogens and the host response to infection. We advance leprosy as a case study due to the sequestering of sufferers in leprosaria and the suggestive skeletal lesions that can result from the disease. Here we present a sequential enzyme extraction protocol, using trypsin followed by ProAlanase, to reduce the abundance of collagen peptides and in so doing increase the detection of non-collagenous proteins. Through our study of five individuals from an 11th to 18th century leprosarium, as well as four from a contemporaneous non-leprosy associated cemetery in Barcelona, we show that samples from 2 out of 5 leprosarium individuals extracted with the sequential digestion methodology contain numerous host immune proteins associated with modern leprosy. In contrast, individuals from the non-leprosy associated cemetery and all samples extracted with a trypsin-only protocol did not. Through this study, we advance a palaeoproteomic methodology to gain insights into the health of archaeological individuals and take a step toward a proteomics-based method to study immune responses in past populations.