Electrical performance of orthotropic and isotropic 3YTZP composites with graphene fillers

3 mol% yttria tetragonal zirconia polycrystal (3YTZP) composites with orthotropic or isotropic microstructures were obtained incorporating few layer graphene (FLG) or exfoliated graphene nanoplatelets (e-GNP) as fillers. Electrical conductivity was studied in a wide range of contents in two configur...

Descripción completa

Detalles Bibliográficos
Autores: López-Pernía, Cristina, Muñoz, Ferreiro, Carmen, Moriche, R., Morales-Rodríguez, Ana, Gallardo-López, Ángela, Poyato, Rosalía
Tipo de recurso: artículo
Estado:Versión publicada
Fecha de publicación:2023
País:España
Institución:Consejo Superior de Investigaciones Científicas (CSIC)
Repositorio:DIGITAL.CSIC. Repositorio Institucional del CSIC
OAI Identifier:oai:digital.csic.es:10261/347692
Acceso en línea:http://hdl.handle.net/10261/347692
https://api.elsevier.com/content/abstract/scopus_id/85143169977
Access Level:acceso abierto
Palabra clave:Zirconia
Aspect ratio
Electrical conductivity
Graphene-based nanostructures (GBN)
Percolation threshold
Descripción
Sumario:3 mol% yttria tetragonal zirconia polycrystal (3YTZP) composites with orthotropic or isotropic microstructures were obtained incorporating few layer graphene (FLG) or exfoliated graphene nanoplatelets (e-GNP) as fillers. Electrical conductivity was studied in a wide range of contents in two configurations: perpendicular (σꓕ) and parallel (σ//) to the pressing axis during spark plasma sintering (SPS). Isotropic e-GNP composites presented excellent electrical conductivity for high e-GNP contents (σꓕ ∼ 3200 S/m and σ// ∼ 1900 S/m for 20 vol% e-GNP), consequence of their misoriented distribution throughout the matrix. Optimum electrical performance was achieved in the highly anisotropic FLG composites, with high electrical conductivity for low contents (σꓕ ∼ 680 S/m for 5 vol%), percolation threshold below 2.5 vol% FLG and outstanding electrical conductivity for high contents (σꓕ ∼ 4000 S/m for 20 vol%), result of the high aspect ratio and low thickness of FLG.