Detection of Nutrients and Contaminants in the Agri-Food Industry Evaluating the Probabilities of False Compliance and False Non-Compliance Through PLS Models and NIR Spectroscopy

NIR spectroscopy has become one of the most prominent techniques in the food industry due to its easy and fast use. Coupled with PLS, it is a well-established method for determining nutrients, contaminants, or adulterants in foods. Nevertheless, it is not common when calculating the capability of de...

Full description

Bibliographic Details
Authors: Castro Reigía, David, García, Iker, Sanllorente Méndez, Silvia, Ortiz Fernández, Mª Cruz, Sarabia Peinador, Luis Antonio
Format: article
Status:Published version
Publication Date:2025
Country:España
Institution:Universidad de Burgos (UBU)
Repository:Repositorio Institucional de la Universidad de Burgos (RIUBU)
OAI Identifier:oai:riubu.ubu.es:10259/10459
Online Access:http://hdl.handle.net/10259/10459
Access Level:Open access
Keyword:PLS Calibration
NIR Spectroscopy
Contaminants
Food adulterants
Capability of detection
Minimun detectable concentration
False positive
False negative
False compliance
False non-compliance
Química analítica
Alimentos
Chemistry, Analytic
Food
Description
Summary:NIR spectroscopy has become one of the most prominent techniques in the food industry due to its easy and fast use. Coupled with PLS, it is a well-established method for determining nutrients, contaminants, or adulterants in foods. Nevertheless, it is not common when calculating the capability of detection or discrimination given a target/permitted value, providing probabilities of false non-compliance (α) or false compliance (β). That is exactly the main purpose of this work, where a single procedure using the accuracy line to evaluate these figures of merit by generalizing ISO 11843 when using NIR-PLS in real scenarios in agri-food industries is shown. Nevertheless, it is a completely general procedure and can be used in any analytical context in which a PLS calibration is applied. As an example of its versatility, several analytical determinations were performed using different common food matrices in the agri-food industry (butter, flour, milk, yogurt, oil, and olives) for the quantification of protein, fat, salt, and two agrochemicals. Some results were a detection capability of 5.2% of fat in milk, 1.20 mg kg−1 for diflufenican, and 2.34 mg kg−1 for piretrin in olives when maximum limits were established at 5%, 0.6 mg kg−1, and 0.5 mg kg−1 respectively. Also, 1.02% for salt in butter and 11.45%, 3.78%, and 2.65% for protein in flour, milk, and yogurt, respectively, were obtained when minimum limits were established at 1.2%, 12%, 4%, and 3% respectively. In all cases α = β = 0.05.