Rational design of a carbon/potassium poly(heptazine imide) heterojunction for enhanced photocatalytic H2 and H2O2 evolution

[EN] We present the rational design of carbon/potassium poly(heptazine imide) (KPHI) heterostructures via one-step salt-melt assisted condensation for efficient photocatalysis. Hybridizing KPHI with an adenine-derived carbonaceous material (Ad-carbon) displayed an outstanding photocatalytic H-2 evol...

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Detalhes bibliográficos
Autores: Pelicano, Christian Mark, Li, Jiaxin, Silva, Ingrid F., Peng, Lu, Tarakina, Nadezda V., Antonietti, Markus, Cabrero-Antonino, Maria, Navalón Oltra, Sergio|||0000-0001-8423-0759, García Gómez, Hermenegildo|||0000-0002-9664-493X
Formato: artículo
Fecha de publicación:2024
País:España
Recursos:Universitat Politècnica de València (UPV)
Repositorio:RiuNet. Repositorio Institucional de la Universitat Politécnica de Valéncia
Idioma:inglés
OAI Identifier:oai:riunet.upv.es:10251/228804
Acesso em linha:https://riunet.upv.es/handle/10251/228804
Access Level:acceso abierto
Palavra-chave:Potassium poly(heptazine imide)
Carbon/KPHI heterostructures
Photocatalytic hydrogen evolution
Electron transfer
Heterojunction interface
Charge separation
Descrição
Resumo:[EN] We present the rational design of carbon/potassium poly(heptazine imide) (KPHI) heterostructures via one-step salt-melt assisted condensation for efficient photocatalysis. Hybridizing KPHI with an adenine-derived carbonaceous material (Ad-carbon) displayed an outstanding photocatalytic H-2 evolution activity (738 mu mol h(-1) g(cat)(-1); with 3 wt% Pt as the cocatalyst) and photocatalytic H2O2 production (3.94 mmol h(-1) g(cat)(-1)). We establish that the Ad-carbon simultaneously operates as an electron acceptor and a photosensitizer based on structural, optical and photo(electro)chemical characterization. Building an intimate heterojunction between the Ad-carbon and KPHI induced spatial charge separation and prolonged the carrier lifetime. From electrocatalysis, we confirmed that coupling Ad-carbon with KPHI enhanced the surface reaction kinetics towards H-2 evolution and O-2 reduction reactions. Moreover, visual evidence of superior charge transport in the hybrid photocatalyst is revealed through the photodeposition of smaller Pt nanoparticles (similar to 7 nm) with uniform distribution on the carbon regions, which also accounts for the increased catalytic activity.