Reversible molecular encapsulation in self-assembled and mechanically locked containers with polar interior

The present thesis work dealt with the study of the polar interiors of self-assembled homocapsules based on aryl-extended calix[4]pyrrole scaffolds, as well as the anisotropic polar interior of a mechanically locked calix[4]arene-calix[4]pyrrole heterocapsule. The properties of the internal cavities...

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Detalles Bibliográficos
Autor: Espelt Ripoll, Mónica
Tipo de recurso: tesis doctoral
Estado:Versión publicada
Fecha de publicación:2013
País:España
Institución:CBUC, CESCA
Repositorio:TDR. Tesis Doctorales en Red
OAI Identifier:oai:www.tdx.cat:10803/275961
Acceso en línea:http://hdl.handle.net/10803/275961
Access Level:acceso abierto
Palabra clave:molecular capsules
host
guest
mechanically locked capsules
hydrogen bonding
self-assembly
clix(4)pyrroles
calix(4)arenes
supramolecular
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Descripción
Sumario:The present thesis work dealt with the study of the polar interiors of self-assembled homocapsules based on aryl-extended calix[4]pyrrole scaffolds, as well as the anisotropic polar interior of a mechanically locked calix[4]arene-calix[4]pyrrole heterocapsule. The properties of the internal cavities of the receptors were probed through the inclusion of different molecules known as guests. Homologous series of aliphatic N-oxides were used in encapsulation experiments to evaluate the size modification and adaptability exhibited by the aromatic cavity enclosed in both systems. Moreover, new super aryl-extended calix[4]pyrroles were synthesized by the elongation of the aromatic walls of aryl-extended calix[4]pyrroles yielding a substantial increased volume of the internal cavity. Additionally, the preparation of an unprecedented calix[4]pyrrole – calix[4]pyrrole molecular container having the two hemispheres mechanically linked was achieved. This capsule features a sizeable increase of its internal volume when compared to the previous calix[4]arene-calix[4]pyrrole molecular container. Both mechanically locked capsules displayed a bis-[2]-catenane topology. Furthermore, the new mechanically locked homo-dimer possesses polar functionalization at the closed ends of both hemispheres.