Development of starch-rich thermoplastic polymers based on mango kernel flour and different plasticizers

[EN] This work reports on the development of starch-rich thermoplastic based formulations produced by using mango kernel flour, avoiding the extraction process of starch from mango kernel to produce these materials. Glycerol, sorbitol and urea at 15 wt% are used as plasticizers to obtain thermoplast...

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Detalles Bibliográficos
Autores: Gómez-Caturla, Jaume|||0000-0001-8680-4509, Ivorra-Martinez, Juan|||0000-0001-8968-4899, Fenollar, Octavio|||0000-0003-4323-7414, Balart, Rafael|||0000-0001-5670-7126, Garcia-Garcia, Daniel|||0000-0002-2520-0186, Dominici, Franco, Puglia, Debora, Torre, Luigi
Tipo de recurso: artículo
Fecha de publicación:2024
País:España
Institución:Universitat Politècnica de València (UPV)
Repositorio:RiuNet. Repositorio Institucional de la Universitat Politécnica de Valéncia
Idioma:inglés
OAI Identifier:oai:riunet.upv.es:10251/220650
Acceso en línea:https://riunet.upv.es/handle/10251/220650
Access Level:acceso abierto
Palabra clave:Thermoplastic starch
Mango kernel flour
Plasticizer
Mechanical properties
Mango kernel starch
09.- Desarrollar infraestructuras resilientes, promover la industrialización inclusiva y sostenible, y fomentar la innovación
12.- Garantizar las pautas de consumo y de producción sostenibles
13.- Tomar medidas urgentes para combatir el cambio climático y sus efectos
Descripción
Sumario:[EN] This work reports on the development of starch-rich thermoplastic based formulations produced by using mango kernel flour, avoiding the extraction process of starch from mango kernel to produce these materials. Glycerol, sorbitol and urea at 15 wt% are used as plasticizers to obtain thermoplastic starch (TPS) formulations by extrusion and injection-moulding processes. Mechanical results show that sorbitol and urea allowed to obtain samples with tensile strength and elongation at break higher than the glycerol-plasticized sample, achieving values of 2.9 MPa of tensile strength and 42% of elongation at break at 53 % RH. These results are supported by field emission scanning electron microscopy (FESEM) micrographs, where a limited concentration of voids was observed in the samples with sorbitol and urea, indicating a better interaction between starch and the plasticizers. Thermogravimetric analysis (TGA) shows that urea and sorbitol increase the thermal stability of TPS in comparison to the glycerol-plasticized sample. Differential scanning calorimetry (DSC) and dynamic-mechanical-thermal analysis (DMTA) verify the increase in stiffness of the sorbitol and urea plasticized TPS and also illustrate an increase in the glass transition temperature of both samples in comparison to the glycerol-plasticized sample. Glass transition temperatures of 45 °C were achieved for the sample with sorbitol.