Hybridization of molecular and graphene materials for CO2 photocatalytic reduction with selectivity control

In the quest for designing efficient and stable photocatalytic materials for CO2 reduction, hybridizing a selective noble-metal-free molecular catalyst and carbon-based light-absorbing materials has recently emerged as a fruitful approach. In this work, we report about Co quaterpyridine complexes co...

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Bibliographic Details
Authors: Ma, Bing, Blanco Fernandez, Matías, Calvillo, Laura, Chen, Lingjing, Chen, Gui, Lau, Tai-Chu, Dražic, Goran, Bonin, Julien, Robert, Marc, Granozzi, Gaetano
Format: article
Publication Date:2021
Country:España
Institution:Universidad Autónoma de Madrid
Repository:Biblos-e Archivo. Repositorio Institucional de la UAM
Language:English
OAI Identifier:oai:repositorio.uam.es:10486/734040
Online Access:https://hdl.handle.net/10486/734040
https://dx.doi.org/10.1021/jacs.1c02250
Access Level:Open access
Keyword:Acetonitrile
carbon dioxide
cobalt compounds
ethanol
graphene
Química
Description
Summary:In the quest for designing efficient and stable photocatalytic materials for CO2 reduction, hybridizing a selective noble-metal-free molecular catalyst and carbon-based light-absorbing materials has recently emerged as a fruitful approach. In this work, we report about Co quaterpyridine complexes covalently linked to graphene surfaces functionalized by carboxylic acid groups. The nanostructured materials were characterized by X-ray photoemission spectroscopy, X-ray absorption spectroscopy, IR and Raman spectroscopies, high-resolution transmission electronmicroscopy and proved to be highly active in the visible-light-driven CO2 catalytic conversion in acetonitrile solutions. Exceptional stabilities (over 200 h of irradiation) were obtained without compromising the selective conversion of CO2 to products (>97%). Most importantly, complete selectivity control could be obtained upon adjusting the experimental conditions: production of CO as the only product was achieved when using aweak acid (phenol or trifluoroethanol) as a co-substrate, while formate was exclusively obtained in solutions of mixed acetonitrile and triethanolamine