Poly-N-Heterocyclic Carbene Ligands with Polyaromatic Linkers. Self-Assembly and Host-Guest Chemistry

In summary, a series of polytopic ligands based on NHC and MIC ligands have been synthesized in this Doctoral Thesis by means of different synthetic routes that gave rise to systems with very sophisticated architectures. A large variety of metal complexes have been formed based on these salt precurs...

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Detalles Bibliográficos
Autor: Mejuto Nieblas, Carmen
Tipo de recurso: tesis doctoral
Estado:Versión publicada
Fecha de publicación:2017
País:España
Institución:CBUC, CESCA
Repositorio:TDR. Tesis Doctorales en Red
OAI Identifier:oai:www.tdx.cat:10803/404306
Acceso en línea:http://hdl.handle.net/10803/404306
http://dx.doi.org/10.6035/14002.2017.532357
Access Level:acceso abierto
Palabra clave:N-Heterocyclic Carbene Ligands
Self-Assembly
Host-Guest Chemistry
Mesoionic Carbene Ligands
Catalysis
Polyaromatic
Química
546
Descripción
Sumario:In summary, a series of polytopic ligands based on NHC and MIC ligands have been synthesized in this Doctoral Thesis by means of different synthetic routes that gave rise to systems with very sophisticated architectures. A large variety of metal complexes have been formed based on these salt precursors that allowed the preparation of homo and heteroleptic mono-, di- and tri-metal complexes with different geometries. The luminescence properties of various imidazolium salts, the catalytic activity of some of the metal complexes obtained, and host-guest molecular recognition studies have been analyzed.