Thermal evaluation of polymorphic transitions in layered hybrid organic-inorganic perovskites for energy storage applications

Layered hybrid organic-inorganic perovskites (LHOIPs) have gained specific attention in applications such as optoelectronics. However, from the thermal perspective, these materials present a high potential for thermal energy storage applications in solid-state due to their heat storage capacity duri...

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Detalles Bibliográficos
Autores: Salgado Pizarro, Rebeca, Navarro-Rivero, M. E., Ding, Y., Barreneche, Camila, Fernández Renna, Ana Inés
Tipo de recurso: artículo
Estado:Versión publicada
Fecha de publicación:2024
País:España
Institución:Universidad de Oviedo (UNIOVI)
Repositorio:Dipòsit Digital de la UB
OAI Identifier:oai:diposit.ub.edu:2445/225073
Acceso en línea:https://hdl.handle.net/2445/225073
Access Level:acceso abierto
Palabra clave:Espectroscòpia Raman
Ciència dels materials
Emmagatzematge d'energia
Raman spectroscopy
Materials science
Storage of energy
Descripción
Sumario:Layered hybrid organic-inorganic perovskites (LHOIPs) have gained specific attention in applications such as optoelectronics. However, from the thermal perspective, these materials present a high potential for thermal energy storage applications in solid-state due to their heat storage capacity during their phase transitions. Here, we evaluate the first-order transition of these materials from the molecular point of view and make a relation with organic size, which is responsible for the ordering-disordering transition. Six LHOIPs have been synthesised, (C12H25N)2CuCl4, (C14H29N)2CuCl4, (C16H33N)2CuCl4, (C12H24N)2MnCl4, (C14H29N)2MnCl4 and (C16H33N)2MnCl4, where the crystal transformation has been evaluated under X-ray diffraction and Raman, and thermal conductivity as well as the thermal expansion have been studied. This work provides a comprehensive evaluation of the disordering phenomenon that is produced during phase transitions