Trajectory statistical analysis of atmospheric transport patterns and trends in precipitation chemistry of a rural site in NE Spain in 1984-2009

The aim of this study is to interpret the variation of precipitation chemistry during the last 25 years in Montseny (NE Spain) by taking into account the main air mass transport routes and emission sources. To this end, trajectory cluster analysis and source-receptor models were applied to an early...

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Detalles Bibliográficos
Autores: Izquierdo Miguel, Rebeca|||0000-0001-5780-4462, Àvila i Castells, Anna|||0000-0002-4137-0839, Alarcón Jordán, Marta
Tipo de recurso: artículo
Fecha de publicación:2012
País:España
Institución:Universitat Autònoma de Barcelona
Repositorio:Dipòsit Digital de Documents de la UAB
Idioma:inglés
OAI Identifier:oai:ddd.uab.cat:147872
Acceso en línea:https://ddd.uab.cat/record/147872
https://dx.doi.org/urn:doi:10.1016/j.atmosenv.2012.07.060
Access Level:acceso abierto
Palabra clave:Back-trajectories
Cluster analysis
Long-range transport
Mediterranean
Precipitation
Source-receptor model
Descripción
Sumario:The aim of this study is to interpret the variation of precipitation chemistry during the last 25 years in Montseny (NE Spain) by taking into account the main air mass transport routes and emission sources. To this end, trajectory cluster analysis and source-receptor models were applied to an early monitoring period (1984-1993) and compared to a more recent one (1998-2009). A decrease of Atlantic advections and increase of African and European air flows was found. Cluster analysis and source-receptor approaches showed that this region is under the influence of natural and anthropogenic sources from the local and long-range scale. Sulphate and H⁺ source areas extended over a vast stretch of central Europe in the early period, but were drastically reduced in the recent period, showing the effectiveness of pollution abatement measures for S. On the other hand, NO₃- sources areas from central Europe strikingly increased. Ship emissions and industrialisation in Eastern Europe and North Africa seem to be acquiring a greater role in the recent period.