Mechanical, Electrical and Magnetic Properties of Ferrogels with Embedded Iron Oxide Nanoparticles Obtained by Laser Target Evaporation: Focus on Multifunctional Biosensor Applications

Hydrogels are biomimetic materials widely used in the area of biomedical engineering and biosensing. Ferrogels (FG) are magnetic composites capable of functioning as magnetic field sensitive transformers and field assisted drug deliverers. FG can be prepared by incorporating magnetic nanoparticles (...

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Autores: Blyakhman, Felix A., Buznikov, Nikita A., Sklyar, Tatyana F., Safronov, Alexander P., Golubeva, Elizaveta V., Svalov, Andrey V., Sokolov, Sergey Yu, Melnikov, Grigory Yu., Orue Goikuria, Iñaki, Kurlyandskaya, Galina V.
Tipo de recurso: artículo
Fecha de publicación:2018
País:España
Institución:Universidad del País Vasco
Repositorio:Addi. Archivo Digital para la Docencia y la Investigación
OAI Identifier:oai:addi.ehu.eus:10810/31967
Acceso en línea:http://hdl.handle.net/10810/31967
Access Level:acceso abierto
Palabra clave:magnetic nanoparticles
magnetic biosensors
ferrogels
magnetic multilayers
giant magnetoimpedance
mechanoelectrical transduction
polyacrylamide ferrogels
maghemite nanoparticles
biomimetic sensors
mi sensor
impedance
model
films
performance
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spelling Mechanical, Electrical and Magnetic Properties of Ferrogels with Embedded Iron Oxide Nanoparticles Obtained by Laser Target Evaporation: Focus on Multifunctional Biosensor ApplicationsBlyakhman, Felix A.Buznikov, Nikita A.Sklyar, Tatyana F.Safronov, Alexander P.Golubeva, Elizaveta V.Svalov, Andrey V.Sokolov, Sergey YuMelnikov, Grigory Yu.Orue Goikuria, IñakiKurlyandskaya, Galina V.magnetic nanoparticlesmagnetic biosensorsferrogelsmagnetic multilayersgiant magnetoimpedancemechanoelectrical transductionpolyacrylamide ferrogelsmaghemite nanoparticlesbiomimetic sensorsmi sensorimpedancemodelfilmsperformanceHydrogels are biomimetic materials widely used in the area of biomedical engineering and biosensing. Ferrogels (FG) are magnetic composites capable of functioning as magnetic field sensitive transformers and field assisted drug deliverers. FG can be prepared by incorporating magnetic nanoparticles (MNPs) into chemically crosslinked hydrogels. The properties of biomimetic ferrogels for multifunctional biosensor applications can be set up by synthesis. The properties of these biomimetic ferrogels can be thoroughly controlled in a physical experiment environment which is much less demanding than biotests. Two series of ferrogels (soft and dense) based on polyacrylamide (PAAm) with different chemical network densities were synthesized by free-radical polymerization in aqueous solution with N, N'-methylene-diacrylamide as a cross-linker and maghemite Fe2O3 MNPs fabricated by laser target evaporation as a filler. Their mechanical, electrical and magnetic properties were comparatively analyzed. We developed a giant magnetoimpedance (MI) sensor prototype with multilayered FeNi-based sensitive elements deposited onto glass or polymer substrates adapted for FG studies. The MI measurements in the initial state and in the presence of FG with different concentrations of MNPs at a frequency range of 1-300 MHz allowed a precise characterization of the stray fields of the MNPs present in the FG. We proposed an electrodynamic model to describe the MI in multilayered film with a FG layer based on the solution of linearized Maxwell equations for the electromagnetic fields coupled with the Landau-Lifshitz equation for the magnetization dynamics.This work was supported in part within the framework of the state task of the Ministry of Education and Science of Russia 3.6121.2017/8.9; RFBR grants 16-08-00609-a, 18-08-00178, and by the ACTIMAT ELKARTEK grant of the Basque Country Government. Selected studies were made at SGIKER Common Services of UPV-EHU and URFU Common Services. We thank I.V. Beketov, A.A. Chlenova, S.O. Volchkov, V.N. Lepalovskij, A.M. Murzakaev and A.A. Svalova for special support.MDPI201920192018info:eu-repo/semantics/articleapplication/pdfhttp://hdl.handle.net/10810/31967reponame:Addi. Archivo Digital para la Docencia y la Investigacióninstname:Universidad del País VascoIngléshttps://www.mdpi.com/1424-8220/18/3/872info:eu-repo/semantics/openAccesshttp://creativecommons.org/licenses/by/3.0/es/This is an open access article distributed under the Creative Commons Attribution License which permits unrestricted use, distribution, and reproduction in any medium, provided the original work is properly cited (CC BY 4.0).Atribución 3.0 Españaoai:addi.ehu.eus:10810/319672026-06-18T09:23:17Z
dc.title.none.fl_str_mv Mechanical, Electrical and Magnetic Properties of Ferrogels with Embedded Iron Oxide Nanoparticles Obtained by Laser Target Evaporation: Focus on Multifunctional Biosensor Applications
title Mechanical, Electrical and Magnetic Properties of Ferrogels with Embedded Iron Oxide Nanoparticles Obtained by Laser Target Evaporation: Focus on Multifunctional Biosensor Applications
spellingShingle Mechanical, Electrical and Magnetic Properties of Ferrogels with Embedded Iron Oxide Nanoparticles Obtained by Laser Target Evaporation: Focus on Multifunctional Biosensor Applications
Blyakhman, Felix A.
magnetic nanoparticles
magnetic biosensors
ferrogels
magnetic multilayers
giant magnetoimpedance
mechanoelectrical transduction
polyacrylamide ferrogels
maghemite nanoparticles
biomimetic sensors
mi sensor
impedance
model
films
performance
title_short Mechanical, Electrical and Magnetic Properties of Ferrogels with Embedded Iron Oxide Nanoparticles Obtained by Laser Target Evaporation: Focus on Multifunctional Biosensor Applications
title_full Mechanical, Electrical and Magnetic Properties of Ferrogels with Embedded Iron Oxide Nanoparticles Obtained by Laser Target Evaporation: Focus on Multifunctional Biosensor Applications
title_fullStr Mechanical, Electrical and Magnetic Properties of Ferrogels with Embedded Iron Oxide Nanoparticles Obtained by Laser Target Evaporation: Focus on Multifunctional Biosensor Applications
title_full_unstemmed Mechanical, Electrical and Magnetic Properties of Ferrogels with Embedded Iron Oxide Nanoparticles Obtained by Laser Target Evaporation: Focus on Multifunctional Biosensor Applications
title_sort Mechanical, Electrical and Magnetic Properties of Ferrogels with Embedded Iron Oxide Nanoparticles Obtained by Laser Target Evaporation: Focus on Multifunctional Biosensor Applications
dc.creator.none.fl_str_mv Blyakhman, Felix A.
Buznikov, Nikita A.
Sklyar, Tatyana F.
Safronov, Alexander P.
Golubeva, Elizaveta V.
Svalov, Andrey V.
Sokolov, Sergey Yu
Melnikov, Grigory Yu.
Orue Goikuria, Iñaki
Kurlyandskaya, Galina V.
author Blyakhman, Felix A.
author_facet Blyakhman, Felix A.
Buznikov, Nikita A.
Sklyar, Tatyana F.
Safronov, Alexander P.
Golubeva, Elizaveta V.
Svalov, Andrey V.
Sokolov, Sergey Yu
Melnikov, Grigory Yu.
Orue Goikuria, Iñaki
Kurlyandskaya, Galina V.
author_role author
author2 Buznikov, Nikita A.
Sklyar, Tatyana F.
Safronov, Alexander P.
Golubeva, Elizaveta V.
Svalov, Andrey V.
Sokolov, Sergey Yu
Melnikov, Grigory Yu.
Orue Goikuria, Iñaki
Kurlyandskaya, Galina V.
author2_role author
author
author
author
author
author
author
author
author
dc.subject.none.fl_str_mv magnetic nanoparticles
magnetic biosensors
ferrogels
magnetic multilayers
giant magnetoimpedance
mechanoelectrical transduction
polyacrylamide ferrogels
maghemite nanoparticles
biomimetic sensors
mi sensor
impedance
model
films
performance
topic magnetic nanoparticles
magnetic biosensors
ferrogels
magnetic multilayers
giant magnetoimpedance
mechanoelectrical transduction
polyacrylamide ferrogels
maghemite nanoparticles
biomimetic sensors
mi sensor
impedance
model
films
performance
description Hydrogels are biomimetic materials widely used in the area of biomedical engineering and biosensing. Ferrogels (FG) are magnetic composites capable of functioning as magnetic field sensitive transformers and field assisted drug deliverers. FG can be prepared by incorporating magnetic nanoparticles (MNPs) into chemically crosslinked hydrogels. The properties of biomimetic ferrogels for multifunctional biosensor applications can be set up by synthesis. The properties of these biomimetic ferrogels can be thoroughly controlled in a physical experiment environment which is much less demanding than biotests. Two series of ferrogels (soft and dense) based on polyacrylamide (PAAm) with different chemical network densities were synthesized by free-radical polymerization in aqueous solution with N, N'-methylene-diacrylamide as a cross-linker and maghemite Fe2O3 MNPs fabricated by laser target evaporation as a filler. Their mechanical, electrical and magnetic properties were comparatively analyzed. We developed a giant magnetoimpedance (MI) sensor prototype with multilayered FeNi-based sensitive elements deposited onto glass or polymer substrates adapted for FG studies. The MI measurements in the initial state and in the presence of FG with different concentrations of MNPs at a frequency range of 1-300 MHz allowed a precise characterization of the stray fields of the MNPs present in the FG. We proposed an electrodynamic model to describe the MI in multilayered film with a FG layer based on the solution of linearized Maxwell equations for the electromagnetic fields coupled with the Landau-Lifshitz equation for the magnetization dynamics.
publishDate 2018
dc.date.none.fl_str_mv 2018
2019
2019
dc.type.none.fl_str_mv info:eu-repo/semantics/article
format article
dc.identifier.none.fl_str_mv http://hdl.handle.net/10810/31967
url http://hdl.handle.net/10810/31967
dc.language.none.fl_str_mv Inglés
language_invalid_str_mv Inglés
dc.relation.none.fl_str_mv https://www.mdpi.com/1424-8220/18/3/872
dc.rights.none.fl_str_mv info:eu-repo/semantics/openAccess
http://creativecommons.org/licenses/by/3.0/es/
Atribución 3.0 España
eu_rights_str_mv openAccess
rights_invalid_str_mv http://creativecommons.org/licenses/by/3.0/es/
Atribución 3.0 España
dc.format.none.fl_str_mv application/pdf
dc.publisher.none.fl_str_mv MDPI
publisher.none.fl_str_mv MDPI
dc.source.none.fl_str_mv reponame:Addi. Archivo Digital para la Docencia y la Investigación
instname:Universidad del País Vasco
instname_str Universidad del País Vasco
reponame_str Addi. Archivo Digital para la Docencia y la Investigación
collection Addi. Archivo Digital para la Docencia y la Investigación
repository.name.fl_str_mv
repository.mail.fl_str_mv
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score 15,301603

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