Suitability of blended ionic liquid-dimethylsulfoxide electrolyte for lithium-oxygen battery

Electrolytes composed of dimethylsulfoxide (DMSO), 1-ethyl-3-methylimidazolium bis(trifluoromethylsulfonyl)imide (EMI TFSI) and LiClO are characterized for application in lithium-oxygen batteries. The increase of EMI TFSI content in the electrolyte enables to improve its thermal stability and to dec...

Descripción completa

Detalles Bibliográficos
Autores: Knipping, Etienne|||0000-0002-0436-5117, Aucher, Christophe|||0000-0002-9455-4156, Guirado, Gonzalo|||0000-0003-2128-7007, Aubouy, Laurent
Tipo de recurso: artículo
Fecha de publicación:2019
País:España
Institución:Universitat Autònoma de Barcelona
Repositorio:Dipòsit Digital de Documents de la UAB
Idioma:inglés
OAI Identifier:oai:ddd.uab.cat:274562
Acceso en línea:https://ddd.uab.cat/record/274562
https://dx.doi.org/urn:doi:10.1002/batt.201800078
Access Level:acceso abierto
Palabra clave:Li-O2 battery
Ionic liquids
Descripción
Sumario:Electrolytes composed of dimethylsulfoxide (DMSO), 1-ethyl-3-methylimidazolium bis(trifluoromethylsulfonyl)imide (EMI TFSI) and LiClO are characterized for application in lithium-oxygen batteries. The increase of EMI TFSI content in the electrolyte enables to improve its thermal stability and to decrease the overpotential of the cell. The optimum addition of EMI TFSI enables to reduce the overpotential from 1.43 V to 1.06 V, with a cyclability of 69 cycles with 600 mAh g of limited capacity.