Spin-texture inversion in the giant Rashba semiconductor BiTeI

Semiconductors with strong spin–orbit interaction as the underlying mechanism for the generation of spin-polarized electrons are showing potential for applications in spintronic devices. Unveiling the full spin texture in momentum space for such materials and its relation to the microscopic structur...

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Detalhes bibliográficos
Autores: Maaß, Henriette, Bentmann, Hendrik, Seibel, Christoph, Tusche, C., Eremeev, Sergey V., Peixoto, T. R. F., Tereshchenko, Oleg E., Kokh, Konstantin A., Chulkov, Eugene V., Kirschner, J., Reinert, Friedrich
Tipo de documento: artigo
Estado:Versão publicada
Data de publicação:2016
País:España
Recursos:Consejo Superior de Investigaciones Científicas (CSIC)
Repositório:DIGITAL.CSIC. Repositorio Institucional del CSIC
OAI Identifier:oai:digital.csic.es:10261/246444
Acesso em linha:http://hdl.handle.net/10261/246444
Access Level:Acceso aberto
Palavra-chave:ddc:537
Descrição
Resumo:Semiconductors with strong spin–orbit interaction as the underlying mechanism for the generation of spin-polarized electrons are showing potential for applications in spintronic devices. Unveiling the full spin texture in momentum space for such materials and its relation to the microscopic structure of the electronic wave functions is experimentally challenging and yet essential for exploiting spin–orbit effects for spin manipulation. Here we employ a state-of-the-art photoelectron momentum microscope with a multichannel spin filter to directly image the spin texture of the layered polar semiconductor BiTeI within the full two-dimensional momentum plane. Our experimental results, supported by relativistic ab initio calculations, demonstrate that the valence and conduction band electrons in BiTeI have spin textures of opposite chirality and of pronounced orbital dependence beyond the standard Rashba model, the latter giving rise to strong optical selection-rule effects on the photoelectron spin polarization. These observations open avenues for spin-texture manipulation by atomic-layer and charge carrier control in polar semiconductors.