Synthesis and structure of [M(CO)4{(PPh2)2CHAu(PPh3)}] (M = Cr, Mo, W)

The reaction of diethyl ether solutions of Li[M(CO)4{(PPh2)2CH}] with [AuCl(PPh3)] gives [M(CO)4{(PPh2)2CHAu(PPh3)}] (M = Cr, Mo, W). The structure of the derivative with M = Mo was determined by single-crystal X-ray diffraction at 173 K. Crystals are monoclinic, space group P22, a = 13.552(3), b =...

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Detalles Bibliográficos
Autores: Fernández, E.J. [0000-0002-6501-744X], Concepción Gimeno, M. [0000-0003-0553-0695], Jones, P.G., Laguna, A. [0000-0003-1984-7538], Laguna, M. [0000-0002-5801-3352], Olmos, E. [0000-0001-8890-8977]
Tipo de recurso: artículo
Estado:Versión publicada
Fecha de publicación:1995
País:España
Institución:Universidad de La Rioja (UR)
Repositorio:RIUR. Repositorio Institucional de la Universidad de La Rioja
OAI Identifier:oai:portal.dialnet.es:doc/5bbc683cb750603269e80514
Acceso en línea:https://investigacion.unirioja.es/documentos/5bbc683cb750603269e80514
Access Level:acceso abierto
Palabra clave:Crystal structures
Gold complexes
Group 6 metal complexes
Tridentate ligand complexes
Descripción
Sumario:The reaction of diethyl ether solutions of Li[M(CO)4{(PPh2)2CH}] with [AuCl(PPh3)] gives [M(CO)4{(PPh2)2CHAu(PPh3)}] (M = Cr, Mo, W). The structure of the derivative with M = Mo was determined by single-crystal X-ray diffraction at 173 K. Crystals are monoclinic, space group P22, a = 13.552(3), b = 17.390(4), c = 17.390(4) A ̊, β = 90.94(2)°, Z = 4 and R(F) = 0.031. The two independent molecules are very similar. The molybdenum and the gold atoms display octahedral and linear geometries, respectively; the shortest intramolecular molybdenum-gold interaction is 4.52 Å. © 1995.