In vitro Corrosion-Assisted Cracking of AZ31B Mg Alloy with a Hybrid PEO-MWCNTs/PCL Coating

The effects of multi-walled carbon nanotubes (MWCNTs) incorporation and polycaprolactone (PCL) post-treatment on the environmental-assisted cracking behaviour of a plasma electrolytic oxidation (PEO) coated AZ31B Mg alloy were elucidated in this study. Slow strain rate tensile (SSRT) experiments wer...

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Detalles Bibliográficos
Autores: Daavari, Morteza, Conde, Ana, Atapour, Masoud, HosseinpourRokni, Mohsen, Mora Sánchez, Hugo, Mohedano Sánchez, Marta, Matykina, Endzhe, Arrabal Durán, Raúl
Tipo de recurso: artículo
Fecha de publicación:2023
País:España
Institución:Universidad Complutense de Madrid (UCM)
Repositorio:Docta Complutense
Idioma:inglés
OAI Identifier:oai:docta.ucm.es:20.500.14352/118074
Acceso en línea:https://hdl.handle.net/20.500.14352/118074
Access Level:acceso abierto
Palabra clave:620
Biodegradable orthopaedic Mg-based implant
Plasma electrolytic oxidation (PEO)
Environmental-assisted cracking
Multi-walled carbon nanotubes (MWCNTs)
Polycaprolactone (PCL)
Materiales
3312 Tecnología de Materiales
Descripción
Sumario:The effects of multi-walled carbon nanotubes (MWCNTs) incorporation and polycaprolactone (PCL) post-treatment on the environmental-assisted cracking behaviour of a plasma electrolytic oxidation (PEO) coated AZ31B Mg alloy were elucidated in this study. Slow strain rate tensile (SSRT) experiments were carried out in simulated body fluid (SBF) for the bare material and different coating systems with and without MWCNTs and PCL overlay. Electrochemical impedance spectroscopy (EIS) and microscopic examinations (SEM and optical) were also conducted to reveal the role of corrosion on the mechanical response. In spite of the significant positive influence of the PEO coatings (with and without MWCNTs) on the bio-electrochemical behaviour of the AZ31B alloy, the environmental-assisted cracking performance was only marginally improved. Furthermore, PEO+MWCNTs/PCL coating system increased the fracture strain of the specimens by 7% compared to the un coated specimens. Based on the SEM and optical micrographs, hydrogen embrittlement was suggested as the main cause of failure of the coated specimens under the in vitro slow strain rate test conditions.