A first insight into the microstructure and crack propagation in novel boron nitride nanosheet/3YTZP composites

In this work, novel 3mol% yttria tetragonal zirconia polycristalline (3YTZP) ceramic composites with boron nitride nanosheets (BNNS) are investigated for the first time. Highly densified composites with 1 and 4vol% BNNS were obtained by spark plasma sintering (SPS) after BNNS synthesis using a solut...

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Detalles Bibliográficos
Autores: Muñoz Ferreiro, Carmen, Morales Rodríguez, Ana, Gallardo López, Ángela María, Poyato Galán, Rosalía
Tipo de recurso: artículo
Estado:Versión publicada
Fecha de publicación:2021
País:España
Institución:Universidad de Sevilla (US)
Repositorio:idUS. Depósito de Investigación de la Universidad de Sevilla
OAI Identifier:oai:idus.us.es:11441/96491
Acceso en línea:https://hdl.handle.net/11441/96491
https://doi.org/10.1016/j.bsecv.2020.02.003
Access Level:acceso abierto
Palabra clave:3YTZP
BN nanosheets
Composite materials
Mechanical properties
Descripción
Sumario:In this work, novel 3mol% yttria tetragonal zirconia polycristalline (3YTZP) ceramic composites with boron nitride nanosheets (BNNS) are investigated for the first time. Highly densified composites with 1 and 4vol% BNNS were obtained by spark plasma sintering (SPS) after BNNS synthesis using a solution exfoliation method and BNNS dispersion into the ceramic powder by ultrasonication. The BNNS presented homogeneous distribution throughout the ceramic matrix and preferential alignment in the plane perpendicular to the pressing axis during SPS. The BNNS incorporation had practically no effect on the Vickers hardness of the material nor on the Young's modulus. Anisotropy in crack development was found in the composite with 4%vol BNNS, together with a mechanism of extensive microcracking. Several energy-absorbing mechanisms during crack propagation, such as crack deflection, crack bridging, crack branching, BNNS pull-out and BNNS debonding, were identified in the composites by a close observation of the indentation-induced fracture paths.