Morphological and magnetic properties of Co nanoparticle thin films grown on Si3N4

The morphological and magnetic properties of Co nanoparticles deposited by triode sputtering on Si3N4 at 550 °C are reported. The nominal thickness of Co ranges from 2 up to 15 nm, and two different capping layers, Au and Pt, are used. The nanoparticles were characterized by x-ray diffraction and at...

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Bibliographic Details
Authors: Presa, B., Matarranz, R., Clavero Pérez, César, García-Martín, José Miguel, Calleja, J. F., Contreras, M. C.
Format: article
Publication Date:2007
Country:España
Institution:Consejo Superior de Investigaciones Científicas (CSIC)
Repository:DIGITAL.CSIC. Repositorio Institucional del CSIC
OAI Identifier:oai:digital.csic.es:10261/12648
Online Access:http://hdl.handle.net/10261/12648
Access Level:Open access
Keyword:Atomic force microscopy
Cobalt
Coercive force
Crystal structures
Ferromagnetic materials
Magnetic anisotropy
Magnetic particles
Magnetic susceptibility
Magnetic thin films
Nanostructured materials
Particle size
Percolation
Sputter deposition
X-ray diffraction
Description
Summary:The morphological and magnetic properties of Co nanoparticles deposited by triode sputtering on Si3N4 at 550 °C are reported. The nominal thickness of Co ranges from 2 up to 15 nm, and two different capping layers, Au and Pt, are used. The nanoparticles were characterized by x-ray diffraction and atomic force microscopy. Morphological and structural studies show that the nanoparticles grow in a well-defined nanostructured pattern and adopt a hexagonal closed packed crystalline structure. Moreover, the average particle size and the particle size dispersion increase as the thickness increases, due to percolation. Experimental characterization of effective anisotropy field was carried out with transverse susceptibility. Transverse susceptibility measurements reveal an in-plane isotropic magnetic behavior. Both the effective anisotropy field and the coercive field increase as the particle size increases, following a D6 dependence, which is typical for three-dimensional structures in the framework of the random anisotropy model. The relationship between the particle size distribution and the anisotropy field distribution is shown, explaining the significant dependence of the magnetic behavior on the Co layer thickness. On the other hand, different capping layers give rise to a change in the magnetic response due to the modification of the interparticle interaction.