Relaxation and derelaxation of pure and hydrogenated amorphous silicon during thermal annealing experiments

The structural relaxation of pure amorphous silicon a-Si and hydrogenated amorphous silicon a-Si:H materials, that occurs during thermal annealing experiments, has been analyzed by Raman spectroscopy and differential scanning calorimetry. Unlike a-Si, the heat evolved from a-Si:H cannot be explained...

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Detalles Bibliográficos
Autores: Kail, F., Farjas Silva, Jordi, Roura Grabulosa, Pere, Secouard, C., Nos Aguilà, Oriol, Bertomeu i Balagueró, Joan, Alzina Sureda, Francesc, Roca i Cabarrocas, P. (Pere)
Tipo de recurso: artículo
Estado:Versión publicada
Fecha de publicación:2010
País:España
Institución:Universidad de Barcelona
Repositorio:Dipòsit Digital de la UB
OAI Identifier:oai:diposit.ub.edu:2445/34662
Acceso en línea:https://hdl.handle.net/2445/34662
Access Level:acceso abierto
Palabra clave:Semiconductors amorfs
Calorimetria
Hidrogen
Silici
Espectroscòpia Raman
Amorphous semiconductors
Calorimetry
Hydrogen
Silicon
Raman spectroscopy
Descripción
Sumario:The structural relaxation of pure amorphous silicon a-Si and hydrogenated amorphous silicon a-Si:H materials, that occurs during thermal annealing experiments, has been analyzed by Raman spectroscopy and differential scanning calorimetry. Unlike a-Si, the heat evolved from a-Si:H cannot be explained by relaxation of the Si-Si network strain but it reveals a derelaxation of the bond angle strain. Since the state of relaxation after annealing is very similar for pure and hydrogenated materials, our results give strong experimental support to the predicted configurational gap between a-Si and crystalline silicon.