Vertical distribution and trace element contamination in sediment cores affected by gold mining in Colombia

The vertical distribution, level of contamination, potential ecological risks, and historical fluxes of trace elements (Pb, As, and Hg) were evaluated from 210Pb-dated sediment cores in three different areas with gold mining impacts in northern Colombia: the Atrato River (AR), the Delicias Marsh (DM...

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Detalles Bibliográficos
Autores: Marrugo-Negrete, José, Pinedo-Hernández, José, Marrugo-Madrid, Siday, Paternina-Uribe, Roberth, Ruiz-Fernández, Ana Carolina, Sánchez-Cabeza, Joan-Albert
Tipo de recurso: artículo
Estado:Versión aceptada para publicación
Fecha de publicación:2023
País:España
Institución:Consejo Superior de Investigaciones Científicas (CSIC)
Repositorio:DIGITAL.CSIC. Repositorio Institucional del CSIC
OAI Identifier:oai:digital.csic.es:10261/334373
Acceso en línea:http://hdl.handle.net/10261/334373
https://api.elsevier.com/content/abstract/scopus_id/85168795401
Access Level:acceso abierto
Palabra clave:Sediment core
Arsenic
Environmental pollution assessment
Gold mining
Lead
Mercury
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Descripción
Sumario:The vertical distribution, level of contamination, potential ecological risks, and historical fluxes of trace elements (Pb, As, and Hg) were evaluated from 210Pb-dated sediment cores in three different areas with gold mining impacts in northern Colombia: the Atrato River (AR), the Delicias Marsh (DM) and the Encaramada Marsh (EM). All cores spanned ∼100 years; the mass accumulation rates followed the order AR > DM > EM. The average trace elements concentrations in the sediment cores were: Pb 2.41 ± 0.72, As 0.65 ± 0.32, Hg 0.07 ± 0.02 μg g-1 in the Atrato River; Pb 23.49 ± 2.59, As 2.46 ± 0.88, Hg 0.10 ± 0.02 μg g-1 in the Delicias Marsh; and Pb 9.76 ± 4.18, As 2.44 ± 1.26, Hg 0.17 ± 0.06 μg g-1 in the Encaramada Marsh. Sediments are classified according to the contamination factor (CF) and geoaccumulation index (Igeo) as low to very highly contaminated. The Pollution load index (PLI) indicates environmental deterioration (PLI> 1), and the Sediment quality guidelines (SQGs) indicate that only Hg may produce adverse biological effects in the EM core. This study is an example of the reconstruction of temporal changes in pollution levels and impacts of potentially toxic elements caused by gold mining in remote ecosystems, which can be reproduced in other areas where environmental monitoring is scarce or non-existent.