Organocatalysis on Tap: Enantioselective Continuous Flow Processes Mediated by Solid-Supported Chiral Organocatalysts

<p style="text-align: justify;"> Sustainability concerns are reshaping the way chemists work, not only at the stage of process design, but also when actually performing reactions. This change of paradigm is exemplified by the deployment of continuous flow techniques, which are slowly...

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Detalhes bibliográficos
Autores: Rodríguez-Escrich, Carles, Pericàs, Miquel A.
Formato: artículo
Fecha de publicación:2015
País:España
Recursos:Varias* (Consorci de Biblioteques Universitáries de Catalunya, Centre de Serveis Científics i Acadèmics de Catalunya)
Repositorio:Recercat. Dipósit de la Recerca de Catalunya
OAI Identifier:oai:recercat.cat:2072/305808
Acesso em linha:http://hdl.handle.net/2072/305808
https://doi.org/10.1002/ejoc.201403042
Access Level:acceso abierto
Palavra-chave:Continuous flow chemistry
Supported catalysts
Asymmetric catalysis
Organocatalysis
Sustainable chemistry
Descrição
Resumo:<p style="text-align: justify;"> Sustainability concerns are reshaping the way chemists work, not only at the stage of process design, but also when actually performing reactions. This change of paradigm is exemplified by the deployment of continuous flow techniques, which are slowly becoming a mainstream practice. Indeed, the possibility of performing catalytic processes (the flagship of sustainable chemistry) in flow presents distinctive advantages. Thus, several authors are focusing their efforts in trying to get the best of these two worlds, with the consequent challenge of finding common solutions for their respective issues. In the last years, this approach has been taken one step further with the use in flow processing of enantioselective organocatalysts, which allow the production of enantiopure compounds free of metal contaminants. Herein, we will cover the literature concerning the use of solid-supported organocatalysts for the continuous flow production of enantiomerically enriched compounds.</p>