New cyclen-cored dendrimers functionalized with pyrene: Synthesis characterization, optical and photophysical properties

New cyclen (1,4,7,10-teraazacyclododecane) cored dendrimers up to the second generation, functionalized with 4, 8 and 16 pyrene units, respectively, were synthesized following a convergent procedure. All new compounds were characterized by NMR spectroscopies and ESI or MALDI TOF mass spectrometry. T...

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Detalhes bibliográficos
Autores: Cevallos Vallejo, Amanda Sofía, Vonlanthen, Mireille, Porcu, Pasquale, Ruiu, Andrea, Rivera, Ernesto
Formato: artículo
Estado:Versión publicada
Fecha de publicación:2017
País:Ecuador
Recursos:Universidad Regional Amazónica
Repositorio:Repositorio Universidad Regional Amazónica
OAI Identifier:oai:repositorio.ikiam.edu.ec:RD_IKIAM/161
Acesso em linha:http://repositorio.ikiam.edu.ec/jspui/handle/RD_IKIAM/161
https://doi.org/10.1016/j.tetlet.2017.02.054
Access Level:acceso abierto
Palavra-chave:Pyrene
Cyclen
Dendrimer
Optical properties
Descrição
Resumo:New cyclen (1,4,7,10-teraazacyclododecane) cored dendrimers up to the second generation, functionalized with 4, 8 and 16 pyrene units, respectively, were synthesized following a convergent procedure. All new compounds were characterized by NMR spectroscopies and ESI or MALDI TOF mass spectrometry. The optical and photophysical properties of the new dendrimers were studied in THF solution. Absorption spectra showed the typical absorption bands of pyrene moieties. In the fluorescence spectra, monomer as well as excimer emission were observed for all compounds. An increased proportion of excimer emission was observed in the dendrimer of the highest generation.