Actividad catalítica de complejos de rodio (I) con ligandos bidentados a base de fósforo en reacciones de hidroformilación de limoneno

We have prepared the com¬plexes RhCl(dppe)2, RhCl(dppp)2 and RhCl(dppb)2, where dppe = diphenylphosphinoethane; dppp = diphenylphosphinopropane; dppb = diphenylphosphinobutane. The above complexes were used as catalytic precursor in the hydroformylation of limonene at differents concentrations and t...

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Detalhes bibliográficos
Autores: Montalvo, Liliana, Bolaños Rivera, Alberto, Cabrera, Armando
Formato: artículo
Estado:Versión publicada
Fecha de publicación:2007
País:Colombia
Recursos:Universidad Autónoma de Occidente
Repositorio:RED: Repositorio Educativo Digital UAO
Idioma:español
OAI Identifier:oai:red.uao.edu.co:10614/174
Acesso em linha:http://hdl.handle.net/10614/174
Access Level:acceso abierto
Palavra-chave:Catálisis homogénea
Rodio
Homogeneous catalysis
Rhodium
Descrição
Resumo:We have prepared the com¬plexes RhCl(dppe)2, RhCl(dppp)2 and RhCl(dppb)2, where dppe = diphenylphosphinoethane; dppp = diphenylphosphinopropane; dppb = diphenylphosphinobutane. The above complexes were used as catalytic precursor in the hydroformylation of limonene at differents concentrations and temperatures. It has found that the best catalytic precursor was the Rhodium complex with dppb as ligand it seems that the P-Rh-P angle is very important in substrate activation