Spatial and temporal distribution of perfluoroalkyl substances (PFAS) detected after an aqueous film forming foam (AFFF) spill

In 2015, > 460,000 L of aqueous film-forming foam (AFFF) and fire suppressors containing per- and polyfluoroalkyl substances (PFAS) were used to combat a fire at a petrochemical fuel storage terminal in the Port of Santos (Brazil). Sediments from seven sites were sampled repeatedly from 2 weeks t...

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Detalles Bibliográficos
Autores: Miranda, Daniele A., Abessa, Denis M.S. [UNESP], Moreira, Lucas B. [UNESP], Maranho, Luciane A. [UNESP], Oliveira, Lauriney G. [UNESP], Benskin, Jonathan P., Leonel, Juliana
Tipo de recurso: artículo
Estado:Versión publicada
Fecha de publicación:2024
País:Brasil
Institución:Universidade Estadual Paulista (UNESP)
Repositorio:Repositório Institucional da UNESP
Idioma:inglés
OAI Identifier:oai:repositorio.unesp.br:11449/309139
Acceso en línea:http://dx.doi.org/10.1016/j.marpolbul.2024.116561
https://hdl.handle.net/11449/309139
Access Level:acceso abierto
Palabra clave:Aqueous film forming foam (AFFF)
PFAS
PFHxA
Santos Estuarine System
Subtropical estuary
Descripción
Sumario:In 2015, > 460,000 L of aqueous film-forming foam (AFFF) and fire suppressors containing per- and polyfluoroalkyl substances (PFAS) were used to combat a fire at a petrochemical fuel storage terminal in the Port of Santos (Brazil). Sediments from seven sites were sampled repeatedly from 2 weeks to 1 year after the fire (n = 30). Ʃ15PFAS concentrations ranged from 115 to 15,931 pg g−1 dry weight (dw). Perfluorooctane sulfonic acid (PFOS) was the most frequently detected compound with concentrations ranging from 363 to 4517 (average = 1603) pg g−1dw to <47.1 to 642 (average = 401) pg g−1 dw, followed by perfluorohexanoic acid (PFHxA) (from 38.8 to 219 (average = 162) pg g−1 dw after 15 days and from <20.8 to 161 (average = 101) pg g−1 dw one year later). Together, the hydrodynamics and fire events documented in the region were important features explaining the spread of PFAS.