ESTRUTURA E PROPRIEDADES ÓPTICAS DO SISTEMA TITANATO-ESTANATO DE ESTRÔNCIO [Sr(Ti1-xSnx)O3 x = 0; 0,25; 0,50; 0,75; 1]

Titanates have perovskite crystalline structure very known for electrical and optical properties used in the electronic devices such as sensors, capacitors, nonvolatile and dynamic random access memories. In particular, titanates structures are characterized for the ABO3 formula being A crystallogra...

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Detalles Bibliográficos
Autor: Inglês, Daniella
Tipo de recurso: tesis de maestría
Estado:Versión publicada
Fecha de publicación:2013
País:Brasil
Institución:Universidade Estadual de Ponta Grossa (UEPG)
Repositorio:Biblioteca Digital de Teses e Dissertações da UEPG
Idioma:portugués
OAI Identifier:oai:tede2.uepg.br:prefix/2109
Acceso en línea:http://tede2.uepg.br/jspui/handle/prefix/2109
Access Level:acceso abierto
Palabra clave:simulação
Teoria do Funcional de Densidade
funcional híbrido
DFT
B3LYP
Perovskita
ABO3
semicondutor
óptico
cerâmica
óxido
titanato-estanato de estrôncio
titanato de estrôncio
estanato de estrôncio
simulation
density functional theory
hybrid functional
Perovskite
semiconductor
optical
ceramics oxide
titanate-strontium stannate
strontium titanate
strontium stannate
CNPQ::CIENCIAS EXATAS E DA TERRA::QUIMICA
Descripción
Sumario:Titanates have perovskite crystalline structure very known for electrical and optical properties used in the electronic devices such as sensors, capacitors, nonvolatile and dynamic random access memories. In particular, titanates structures are characterized for the ABO3 formula being A crystallographic site formed by 12 atoms neighbors and B crystallographic site formed by 6 atoms neighbors. However, researches about strontium titanate-stannate system are found minimally in the literature. Articles discussing synthesis, characterization and compositions are insufficiently presented. This project shows a theoretical study of the structure and optical properties of the strontium titanate-stannate system for different substitutions [Sr(Ti1-xSnx)O3 x = 0; 0,25; 0,50; 0,75; 1]. It was used theoretical-computational methodology based on, Density Functional Theory (DFT) with B3LYP functional to calculate the structure of the models SrTiO3 (STO), Sr(Ti1-xSnx)O3 (STS) and SrSnO3 (SSO). Theoretical data of parameter lattice, cell unit angles, volume, band gap, overlap population, charges and free energy are presented as well as analysis and discussion of the results for band structure (EB), density of states (DOS), electron density maps. Thus, one may present the data obtained and investigate the properties of the materials.