The new psychoactive substances 25H-NBOMe and 25H-NBOH induce abnormal development in the zebrafish embryo and interact in the DNA major groove

Toxicological effects of 25H-NBOMe and 25H-NBOH recreational drugs on zebrafish embryos and larvae at the end of 96 h exposure period were demonstrated. 25H-NBOH and 25H-NBOMe caused high embryo mortality at 80 and 100 µg mL−1, respectively. According to the decrease in the concentration tested, let...

Descripción completa

Detalles Bibliográficos
Autores: Wellington Alves de Barros, Ângelo de Fátima, Camila da Silva Nunes, Juliana Alves da Costa Ribeiro Souza, Igor José dos Santos Nascimento, Isis Martins Figueiredo, Thiago Mendonça de Aquino, Leonardo Vieira, Davi Felipe Farias, Josué Carinhanha Caldas Santos
Tipo de recurso: artículo
Estado:Versión publicada
Fecha de publicación:2021
País:Brasil
Institución:Universidade Federal de Minas Gerais (UFMG)
Repositorio:Repositório Institucional da UFMG
Idioma:inglés
OAI Identifier:oai:repositorio.ufmg.br:1843/77990
Acceso en línea:https://doi.org/10.1016/j.crtox.2021.11.002
http://hdl.handle.net/1843/77990
https://orcid.org/0000-0002-3479-0720
https://orcid.org/0000-0003-2344-5590
https://orcid.org/0000-0002-2664-4336
https://orcid.org/0000-0002-1873-5342
https://orcid.org/0000-0001-9138-8466
https://orcid.org/0000-0002-9525-5123
https://orcid.org/0000-0001-5438-1919
Access Level:acceso abierto
Palabra clave:Phenethylamines
Ilicit Drugs
DNA interaction
Zebra fish
NBOHs
NBOMes
Drogas - Toxicologia
Fenetilamina
Drogas - Uso recreativo
DNA
Alucinógenos
Espectroscopia de fluorescência
Espectroscopia de ressonância nuclear
Descripción
Sumario:Toxicological effects of 25H-NBOMe and 25H-NBOH recreational drugs on zebrafish embryos and larvae at the end of 96 h exposure period were demonstrated. 25H-NBOH and 25H-NBOMe caused high embryo mortality at 80 and 100 µg mL−1, respectively. According to the decrease in the concentration tested, lethality decreased while non-lethal effects were predominant up to 10 and 50 µg mL−1 of 25H-NBOH and 25H-NBOMe, respectively, including spine malformation, egg hatching delay, body malformation, otolith malformation, pericardial edema, and blood clotting. We can disclose that these drugs have an affinity for DNA in vitro using biophysical spectroscopic assays and molecular modeling methods. The experiments demonstrated that 25H-NBOH and 25H-NBOMe bind to the unclassical major groove of ctDNA with a binding constant of 27.00 × 104 M−1 and 5.27 × 104 M−1, respectively. Furthermore, these interactions lead to conformational changes in the DNA structure. Therefore, the results observed in the zebrafish embryos and DNA may be correlated.