Microestrutura e propriedades mecânicas de vitrocerâmicos do sistema Li2O – CaO – SiO2

An interesting characteristic of the Li2O-CaO-SiO2 glass-forming system is the possibility of obtaining certain crystalline phases and morphologies that may lead to tough glass-ceramics. However, very few published works investigated this matter. Glass compositions within the range 30-50% CaSiO3 / 7...

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Detalles Bibliográficos
Autor: Santos, Gisele Guimarães dos
Tipo de recurso: tesis de maestría
Estado:Versión publicada
Fecha de publicación:2013
País:Brasil
Institución:Universidade Federal de São Carlos (UFSCAR)
Repositorio:Repositório Institucional da UFSCAR
Idioma:portugués
OAI Identifier:oai:repositorio.ufscar.br:20.500.14289/10241
Acceso en línea:https://repositorio.ufscar.br/handle/20.500.14289/10241
Access Level:acceso abierto
Palabra clave:Vidro
Vitrocerâmica
Cristalização
Microestrutura
Propriedades mecânicas
Glass
Crystallization
Microstructure
Mechanical properties
ENGENHARIAS::ENGENHARIA DE MATERIAIS E METALURGICA
Descripción
Sumario:An interesting characteristic of the Li2O-CaO-SiO2 glass-forming system is the possibility of obtaining certain crystalline phases and morphologies that may lead to tough glass-ceramics. However, very few published works investigated this matter. Glass compositions within the range 30-50% CaSiO3 / 70-50% Li2SiO3 were studied to obtain appropriate microstructures. Heat treatments were conducted using the double treatment technique: nucleation at about the glass transition temperature followed by crystal growth within the temperature range 500 and 700°C. These temperatures were selected according to DSC data. The influence of the size, number and morphology of the crystals on certain mechanical properties of the glass-ceramics, such as hardness and indentation toughness, were estimated by Vickers indentation tests. The samples were also characterized by X-ray diffraction to identify the phases present and by MEV to examine the crystal size, percentage and morphology. The best results were obtained with a composition of 44% mol CaSiO3 using the following thermal treatment conditions: 498°C for 24 hours (nucleation) and 700°C for 2 hours (Crystal growth), that led to a glass-ceramic showing a toughness of 1,9 MPa.m1/2.