Thermal study and characterization of new cocrystals of ciprofloxacin with picolinic acid

This article describes the mechanochemical synthesis (liquid-assisted grinding (LAG) and neat grinding (NG)), characterization and thermoanalytical study of new cocrystals of ciprofloxacin (CIP) with picolinic acid (PCA) in a 1:1 molar ratio. Characterization was performed through thermoanalytical t...

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Detalles Bibliográficos
Autores: Torquetti, Carolina [UNESP], Ferreira, Patrícia Osório [UNESP], de Almeida, Amanda Cosmo [UNESP], Fernandes, Richard Perosa [UNESP], Caires, Flávio Junior [UNESP]
Tipo de recurso: artículo
Estado:Versión publicada
Fecha de publicación:2021
País:Brasil
Institución:Universidade Estadual Paulista (UNESP)
Repositorio:Repositório Institucional da UNESP
Idioma:inglés
OAI Identifier:oai:repositorio.unesp.br:11449/205850
Acceso en línea:http://dx.doi.org/10.1007/s10973-020-10479-3
http://hdl.handle.net/11449/205850
Access Level:acceso abierto
Palabra clave:Ciprofloxacin
Coamorphous
Cocrystal
Cocrystal solvate
Mechanochemistry
Thermal analysis
Descripción
Sumario:This article describes the mechanochemical synthesis (liquid-assisted grinding (LAG) and neat grinding (NG)), characterization and thermoanalytical study of new cocrystals of ciprofloxacin (CIP) with picolinic acid (PCA) in a 1:1 molar ratio. Characterization was performed through thermoanalytical techniques (differential scanning calorimetry (DSC), simultaneous thermogravimetry and differential scanning calorimetry (TG-DSC)), X-ray powder diffraction (XRPD) and infrared spectroscopy (IR). The thermoanalytical study, together with the XRPD and IR techniques, confirmed the formation of new cocrystal and helped to understand its formation. From the LAG method, using ethanol as a solvent, a cocrystal solvate was obtained. The NG method, together with thermal stress, favored obtaining the cocrystal through a coamorphous intermediate phase. Solubility study of all new materials showed an increase in CIP concentration for the cocrystals compared to pure drug.