Density, viscosity and excess properties of binary mixtures of protic ionic liquid (2-HDEAF, 2-HDEAA) + water at different temperatures

Over the last decade, ionic liquids (IL) have attracted considerable attention for their potential to replace traditional volatile organic solvents due to their well-known physico-chemistry properties. This is an important topic for industrial applications today, and have been the subject of extensi...

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Detalhes bibliográficos
Autores: Pinheiro, Regiane Silva, Mesquita, Francisca Maria Rodrigues, Feitosa, Filipe Xavier, Sant'Ana, Hosiberto Batista de, Aguiar, Rílvia Saraiva de Santiago
Tipo de documento: artigo
Estado:Versão publicada
Data de publicação:2018
País:Brasil
Recursos:Universidade Federal do Ceará (UFC)
Repositório:Repositório Institucional da Universidade Federal do Ceará (UFC)
Idioma:inglês
OAI Identifier:oai:repositorio.ufc.br:riufc/68536
Acesso em linha:http://www.repositorio.ufc.br/handle/riufc/68536
Access Level:Acceso aberto
Palavra-chave:Density
Viscosity
Excess properties
Protic ionic liquid
Descrição
Resumo:Over the last decade, ionic liquids (IL) have attracted considerable attention for their potential to replace traditional volatile organic solvents due to their well-known physico-chemistry properties. This is an important topic for industrial applications today, and have been the subject of extensive literature studies. Nevertheless, there is still a lack of experimental thermodynamics data on aqueous mixtures, i.e., ionic liquids + water, especially volumetric and transport properties. These data could provide essential information about interactions and molecular phenomena in such mixtures. To investigate volumetric and transport properties for ionic liquids + water, density and viscosity data of the protic ionic liquids 2-hydroxydiethanolamine formate (2-HDEAF), 2-hydroxydiethanolamine acetate (2-HDEAA), water and their binary mixtures were measured at T = (293.15 to 343.15) K and atmospheric pressure. Excess molar volumes and deviation of viscosity were computed from experimental density and viscosity values and were fit to the Redlich-Kister equation. We observed a negative behavior for both ionic liquids + water mixtures that can be attributed to a shrinkage of the mixtures.