Proton conduction mechanisms in GPTMS/TEOS-derived organic/silica hybrid films prepared by sol-gel process

In this work, we employed impedance spectroscopy measurements to investigate the electrical properties of hybrid films obtained with the sol-gel process using 3-glycidoxypropyltrimethoxysilane (GPTMS) and tetraethylorthosilicate (TEOS) at different GPTMS/TEOS molar ratios and temperatures of thermal...

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Detalles Bibliográficos
Autores: Monteiro, Daniela A. [UNESP], Gozzi, Giovani [UNESP], Chinaglia, Dante Luis [UNESP], Oliveira, Osvaldo N., de Vicente, Fabio S. [UNESP]
Tipo de recurso: artículo
Estado:Versión publicada
Fecha de publicación:2020
País:Brasil
Institución:Universidade Estadual Paulista (UNESP)
Repositorio:Repositório Institucional da UNESP
Idioma:inglés
OAI Identifier:oai:repositorio.unesp.br:11449/201845
Acceso en línea:http://dx.doi.org/10.1016/j.synthmet.2020.116448
http://hdl.handle.net/11449/201845
Access Level:acceso abierto
Palabra clave:Conduction mechanisms
Epoxy polymerization
Impedance spectroscopy
Organic/silica hybrids
Proton conductivity
Sol-gel
Descripción
Sumario:In this work, we employed impedance spectroscopy measurements to investigate the electrical properties of hybrid films obtained with the sol-gel process using 3-glycidoxypropyltrimethoxysilane (GPTMS) and tetraethylorthosilicate (TEOS) at different GPTMS/TEOS molar ratios and temperatures of thermal treatment. For the GPTMS/TEOS-derived samples with 1:1 composition, the DC conductivity (σdc) and charge carrier mobility (μdc) increased linearly with heat treatment temperature from 25 to 80 °C, while σdc increased from 3.2 to 22.4 nS/cm with a 7-fold increase in the GPTMS concentration. These results could be rationalized with the Miller-Abraham model using a charge carrier activation energy of 0.54 ± 0.03 eV. Using FTIR spectroscopy we demonstrated that the structural arrangement of the hybrid matrix involves epoxy ring opening, thus favoring proton conduction, which occurs as in the Grotthuss mechanism via hopping between nearest oxygen atoms of polymerized glycidoxypropyl groups. It is significant that electrical properties of organic/silica matrices can be predicted and tuned for tailored applications using the modeling presented here.