β-cyclodextrin PAMAM Dendrimer Surface Doped with Silver and Hexacyanoferrate (III) and its Applications for Dopamine Detection in Synthetic Samples

A synthesis of β-cyclodextrin (β-Cd) functionalized with polyamide dendrimer PAMAM G.0 complexed with silver and potassium hexacyanoferrate (III) forming a mixed-valence complex (β-Cd-PAMAM-Ag/Fe) was proposed. This material was characterized by scanning electron microscopy (SEM), infrared spectrosc...

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Detalles Bibliográficos
Autores: Barbosa, Priscila Fernanda Pereira [UNESP], Mastelaro, Valmor Roberto, Vieira, Eduardo Guimarães, Carmo, Devaney Ribeiro do [UNESP]
Tipo de recurso: artículo
Estado:Versión publicada
Fecha de publicación:2022
País:Brasil
Institución:Universidade Estadual Paulista (UNESP)
Repositorio:Repositório Institucional da UNESP
Idioma:inglés
OAI Identifier:oai:repositorio.unesp.br:11449/240126
Acceso en línea:http://dx.doi.org/10.1002/elan.202100628
http://hdl.handle.net/11449/240126
Access Level:acceso abierto
Palabra clave:Cyclodextrin
Dendrimer
Dopamine
Electrochemical measurements
Hexacyanoferrate (III)
Silver
Descripción
Sumario:A synthesis of β-cyclodextrin (β-Cd) functionalized with polyamide dendrimer PAMAM G.0 complexed with silver and potassium hexacyanoferrate (III) forming a mixed-valence complex (β-Cd-PAMAM-Ag/Fe) was proposed. This material was characterized by scanning electron microscopy (SEM), infrared spectroscopy (FT-IR), X-Ray diffraction (XRD), Energy Dispersion Spectroscopy (EDS) and Electron Paramagnetic Resonance (EPR). The hybrid complex was electrochemically investigated using cyclic voltammetry and some parameters (electrolyte, concentration of electrolyte, pH and scan rate) were evaluate in order to obtain optimum analytical responses. The β-Cd-PAMAM-Ag/Fe material was successfully applied in the electrocatalytic oxidation of dopamine (DOP) using Cyclic Voltammetry (CV) and Square Wave Voltammetry (SWV).