Experimental procedure for kinetic studies on egg-shell catalystsThe case of liquid-phase hydrogenation of 1,3-butadiene and n-butenes on commercial Pd catalysts

A study of the liquid-phase hydrogenation of 1,3-butadiene on commercial Pd/Al2O3 catalysts of the “egg-shell” type has been performed. Experimental conditions (40◦C, 4 atm and high conversion of the di-olefin) were selected in accordance to industrial operating conditions employed for selective hyd...

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Detalles Bibliográficos
Autores: Ardiaca, Nestor O., Bressa, Sergio Patricio, Alves, Javier Alberto, Martinez, Osvaldo Miguel, Barreto, Guillermo Fernando
Tipo de recurso: artículo
Estado:Versión publicada
Fecha de publicación:2001
País:Argentina
Institución:Consejo Nacional de Investigaciones Científicas y Técnicas
Repositorio:CONICET Digital (CONICET)
Idioma:inglés
OAI Identifier:oai:ri.conicet.gov.ar:11336/45066
Acceso en línea:http://hdl.handle.net/11336/45066
Access Level:acceso abierto
Palabra clave:Multiphase Reactions
Selective Hydrogenation
Laboratory Reactors
1,3-Butadiene
Pd/Al2o3 Catalyst
https://purl.org/becyt/ford/2.4
https://purl.org/becyt/ford/2
Descripción
Sumario:A study of the liquid-phase hydrogenation of 1,3-butadiene on commercial Pd/Al2O3 catalysts of the “egg-shell” type has been performed. Experimental conditions (40◦C, 4 atm and high conversion of the di-olefin) were selected in accordance to industrial operating conditions employed for selective hydrogenation of 1,3-butadiene. Three experimental schemes were tested: a slurry reactor, a rotating-basket reactor, and a recirculation system with an external fixed-bed reactor. Significant drawbacks shown by the two former devices were mainly derived from the very high activity and the egg-shell structure of the catalysts. Instead, the recirculation system was found to be an excellent alternative. Although Pd is present only within a very thin external layer (around 50–250mm), strong diffusion effects impairing selectivity were observed. Plausible kinetic expressions corresponding to nine series–parallel overall reactions are derived from a mechanistic model. To deal with this network of fast reactions, a rather complex set of computational and predictive tools were employed. A worked out example from several replicates demonstrates the capability of both, experimental and data analysis procedures, for inferring kinetic parameters of the proposed model.