Stacked wire-mesh monoliths for VOCs combustion: Effect of the mesh-opening in the catalytic performance

Structured reactors based on low cost metallic wire-mesh substrates of highly enhanced transport properties can be an interesting alternative to parallel channel monolithic reactors. In this work stacked wire-mesh monoliths were studied for volatile organic compounds elimination. Monoliths of differ...

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Detalles Bibliográficos
Autores: Sanz, Oihane, Banus, Ezequiel David, Goya, Aintzane, Larumbe, Haizea, Delgado, Juan José, Monzón, Antonio, Montes, Mario
Tipo de recurso: artículo
Estado:Versión publicada
Fecha de publicación:2017
País:Argentina
Institución:Consejo Nacional de Investigaciones Científicas y Técnicas
Repositorio:CONICET Digital (CONICET)
Idioma:inglés
OAI Identifier:oai:ri.conicet.gov.ar:11336/43101
Acceso en línea:http://hdl.handle.net/11336/43101
Access Level:acceso abierto
Palabra clave:Vocs Abatement
Pt/Oms-2
Wire-Mesh Monoliths
Mesh-Opening
https://purl.org/becyt/ford/2.4
https://purl.org/becyt/ford/2
Descripción
Sumario:Structured reactors based on low cost metallic wire-mesh substrates of highly enhanced transport properties can be an interesting alternative to parallel channel monolithic reactors. In this work stacked wire-mesh monoliths were studied for volatile organic compounds elimination. Monoliths of different mesh-opening were homogeneously and adherently dip-coated with Pt/Manganese Octahedral Molecular Sieve (OMS-2) bifunctional catalyst. The catalytic activity was tested in toluene and methanol complete oxidation reactions. Catalytic activity increases using stacked wire-mesh monoliths instead of parallel channel monoliths and decreases when increasing the wire-mesh opening, showing the importance of the mass-transfer phenomena (contact between the gas phase and the solid catalyst).