Organocatalysis and Biocatalysis Hand in Hand: Combining Catalysts in One-Pot Procedures

Multi-step processes catalysed by several catalysts working concurrently have been developed in nature, thus improving reaction efficiency. The quest for novel and improved catalytic systems has led to the development of biocatalytic and later to organocatalytic procedures as very valuable tools in...

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Authors: Bisogno, Fabricio Román, López Vidal, Martín Guillermo, de Gonzalo, Gonzalo
Format: article
Status:Published version
Publication Date:2017
Country:Argentina
Institution:Consejo Nacional de Investigaciones Científicas y Técnicas
Repository:CONICET Digital (CONICET)
Language:English
OAI Identifier:oai:ri.conicet.gov.ar:11336/63770
Online Access:http://hdl.handle.net/11336/63770
Access Level:Open access
Keyword:CONCURRENT PROCESSES
ENANTIOSELECTIVITY
ENZYME CATALYSIS
MULTISTEP SYNTHESIS
ONE-POT PROCEDURES
ORGANIC CATALYSIS
https://purl.org/becyt/ford/1.4
https://purl.org/becyt/ford/1
https://purl.org/becyt/ford/2.9
https://purl.org/becyt/ford/2
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spelling Organocatalysis and Biocatalysis Hand in Hand: Combining Catalysts in One-Pot ProceduresBisogno, Fabricio RománLópez Vidal, Martín Guillermode Gonzalo, GonzaloCONCURRENT PROCESSESENANTIOSELECTIVITYENZYME CATALYSISMULTISTEP SYNTHESISONE-POT PROCEDURESORGANIC CATALYSIShttps://purl.org/becyt/ford/1.4https://purl.org/becyt/ford/1https://purl.org/becyt/ford/2.9https://purl.org/becyt/ford/2Multi-step processes catalysed by several catalysts working concurrently have been developed in nature, thus improving reaction efficiency. The quest for novel and improved catalytic systems has led to the development of biocatalytic and later to organocatalytic procedures as very valuable tools in asymmetric synthesis while using mild reaction conditions in the absence of metal catalysts. As a timeless challenge, chemists are facing the need for process designs in which different sorts of catalysts can operate successfully in a one-pot concurrent fashion. Likewise, such designs bring about the best of each catalyst and, in certain cases, enable us to improve problematic issues, such as reactivity, selectivity, solubility, inhibition, etc. Specifically, to combine these two types of catalysts in one-pot, achieving high yields and selectivity, is a fascinating aspect of catalysis. This review covers representative advances in this field, in particular those in which biocatalysts and organocatalysts are employed either in sequential reactions or in simultaneous processes. (Figure presented.).Fil: Bisogno, Fabricio Román. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico Conicet - Córdoba. Instituto de Investigaciones en Físico-química de Córdoba. Universidad Nacional de Córdoba. Facultad de Ciencias Químicas. Instituto de Investigaciones en Físico-química de Córdoba; ArgentinaFil: López Vidal, Martín Guillermo. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico Conicet - Córdoba. Instituto de Investigaciones en Físico-química de Córdoba. Universidad Nacional de Córdoba. Facultad de Ciencias Químicas. Instituto de Investigaciones en Físico-química de Córdoba; ArgentinaFil: de Gonzalo, Gonzalo. Universidad de Sevilla; EspañaWiley VCH Verlag2017-06info:eu-repo/semantics/articleinfo:eu-repo/semantics/publishedVersionhttp://purl.org/coar/resource_type/c_6501info:ar-repo/semantics/articuloapplication/pdfapplication/pdfhttp://hdl.handle.net/11336/63770Bisogno, Fabricio Román; López Vidal, Martín Guillermo; de Gonzalo, Gonzalo; Organocatalysis and Biocatalysis Hand in Hand: Combining Catalysts in One-Pot Procedures; Wiley VCH Verlag; Advanced Synthesis & Catalysis (print); 359; 12; 6-2017; 2026-20491615-4150CONICET DigitalCONICETenginfo:eu-repo/semantics/altIdentifier/doi/10.1002/adsc.201700158info:eu-repo/semantics/altIdentifier/url/https://onlinelibrary.wiley.com/doi/abs/10.1002/adsc.201700158info:eu-repo/semantics/openAccesshttps://creativecommons.org/licenses/by-nc-sa/2.5/ar/reponame:CONICET Digital (CONICET)instname:Consejo Nacional de Investigaciones Científicas y Técnicas2024-05-08T14:18:06Zoai:ri.conicet.gov.ar:11336/63770instacron:CONICETInstitucionalhttp://ri.conicet.gov.ar/Organismo científico-tecnológicoNo correspondehttp://ri.conicet.gov.ar/oai/requestdasensio@conicet.gov.ar; lcarlino@conicet.gov.arArgentinaNo correspondeNo correspondeNo correspondeopendoar:34982024-05-08 14:18:06.512CONICET Digital (CONICET) - Consejo Nacional de Investigaciones Científicas y Técnicasfalse
dc.title.none.fl_str_mv Organocatalysis and Biocatalysis Hand in Hand: Combining Catalysts in One-Pot Procedures
title Organocatalysis and Biocatalysis Hand in Hand: Combining Catalysts in One-Pot Procedures
spellingShingle Organocatalysis and Biocatalysis Hand in Hand: Combining Catalysts in One-Pot Procedures
Bisogno, Fabricio Román
CONCURRENT PROCESSES
ENANTIOSELECTIVITY
ENZYME CATALYSIS
MULTISTEP SYNTHESIS
ONE-POT PROCEDURES
ORGANIC CATALYSIS
https://purl.org/becyt/ford/1.4
https://purl.org/becyt/ford/1
https://purl.org/becyt/ford/2.9
https://purl.org/becyt/ford/2
title_short Organocatalysis and Biocatalysis Hand in Hand: Combining Catalysts in One-Pot Procedures
title_full Organocatalysis and Biocatalysis Hand in Hand: Combining Catalysts in One-Pot Procedures
title_fullStr Organocatalysis and Biocatalysis Hand in Hand: Combining Catalysts in One-Pot Procedures
title_full_unstemmed Organocatalysis and Biocatalysis Hand in Hand: Combining Catalysts in One-Pot Procedures
title_sort Organocatalysis and Biocatalysis Hand in Hand: Combining Catalysts in One-Pot Procedures
dc.creator.none.fl_str_mv Bisogno, Fabricio Román
López Vidal, Martín Guillermo
de Gonzalo, Gonzalo
author Bisogno, Fabricio Román
author_facet Bisogno, Fabricio Román
López Vidal, Martín Guillermo
de Gonzalo, Gonzalo
author_role author
author2 López Vidal, Martín Guillermo
de Gonzalo, Gonzalo
author2_role author
author
dc.subject.none.fl_str_mv CONCURRENT PROCESSES
ENANTIOSELECTIVITY
ENZYME CATALYSIS
MULTISTEP SYNTHESIS
ONE-POT PROCEDURES
ORGANIC CATALYSIS
https://purl.org/becyt/ford/1.4
https://purl.org/becyt/ford/1
https://purl.org/becyt/ford/2.9
https://purl.org/becyt/ford/2
topic CONCURRENT PROCESSES
ENANTIOSELECTIVITY
ENZYME CATALYSIS
MULTISTEP SYNTHESIS
ONE-POT PROCEDURES
ORGANIC CATALYSIS
https://purl.org/becyt/ford/1.4
https://purl.org/becyt/ford/1
https://purl.org/becyt/ford/2.9
https://purl.org/becyt/ford/2
description Multi-step processes catalysed by several catalysts working concurrently have been developed in nature, thus improving reaction efficiency. The quest for novel and improved catalytic systems has led to the development of biocatalytic and later to organocatalytic procedures as very valuable tools in asymmetric synthesis while using mild reaction conditions in the absence of metal catalysts. As a timeless challenge, chemists are facing the need for process designs in which different sorts of catalysts can operate successfully in a one-pot concurrent fashion. Likewise, such designs bring about the best of each catalyst and, in certain cases, enable us to improve problematic issues, such as reactivity, selectivity, solubility, inhibition, etc. Specifically, to combine these two types of catalysts in one-pot, achieving high yields and selectivity, is a fascinating aspect of catalysis. This review covers representative advances in this field, in particular those in which biocatalysts and organocatalysts are employed either in sequential reactions or in simultaneous processes. (Figure presented.).
publishDate 2017
dc.date.none.fl_str_mv 2017-06
dc.type.none.fl_str_mv info:eu-repo/semantics/article
info:eu-repo/semantics/publishedVersion
http://purl.org/coar/resource_type/c_6501
info:ar-repo/semantics/articulo
format article
status_str publishedVersion
dc.identifier.none.fl_str_mv http://hdl.handle.net/11336/63770
Bisogno, Fabricio Román; López Vidal, Martín Guillermo; de Gonzalo, Gonzalo; Organocatalysis and Biocatalysis Hand in Hand: Combining Catalysts in One-Pot Procedures; Wiley VCH Verlag; Advanced Synthesis & Catalysis (print); 359; 12; 6-2017; 2026-2049
1615-4150
CONICET Digital
CONICET
url http://hdl.handle.net/11336/63770
identifier_str_mv Bisogno, Fabricio Román; López Vidal, Martín Guillermo; de Gonzalo, Gonzalo; Organocatalysis and Biocatalysis Hand in Hand: Combining Catalysts in One-Pot Procedures; Wiley VCH Verlag; Advanced Synthesis & Catalysis (print); 359; 12; 6-2017; 2026-2049
1615-4150
CONICET Digital
CONICET
dc.language.none.fl_str_mv eng
language eng
dc.relation.none.fl_str_mv info:eu-repo/semantics/altIdentifier/doi/10.1002/adsc.201700158
info:eu-repo/semantics/altIdentifier/url/https://onlinelibrary.wiley.com/doi/abs/10.1002/adsc.201700158
dc.rights.none.fl_str_mv info:eu-repo/semantics/openAccess
https://creativecommons.org/licenses/by-nc-sa/2.5/ar/
eu_rights_str_mv openAccess
rights_invalid_str_mv https://creativecommons.org/licenses/by-nc-sa/2.5/ar/
dc.format.none.fl_str_mv application/pdf
application/pdf
dc.publisher.none.fl_str_mv Wiley VCH Verlag
publisher.none.fl_str_mv Wiley VCH Verlag
dc.source.none.fl_str_mv reponame:CONICET Digital (CONICET)
instname:Consejo Nacional de Investigaciones Científicas y Técnicas
instname_str Consejo Nacional de Investigaciones Científicas y Técnicas
reponame_str CONICET Digital (CONICET)
collection CONICET Digital (CONICET)
repository.name.fl_str_mv CONICET Digital (CONICET) - Consejo Nacional de Investigaciones Científicas y Técnicas
repository.mail.fl_str_mv dasensio@conicet.gov.ar; lcarlino@conicet.gov.ar
_version_ 1799196188627435520
score 15.812429

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