Electrochemical characterization of MWCNT Ni(OH)₂ composites as cathode materials

The hydrothermal method was used to synthesize multi-walled carbon nanotube/nickel hydroxide composites (MWCNT/Ni(OH)<sub>2</sub>). The structure and morphology of the prepared materials were characterized by X-ray diffraction and transmission electron microscopy. The electrochemical per...

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Detalhes bibliográficos
Autores: Ortiz, Mariela, Real, Silvia Graciela, Castro, Élida Beatriz
Tipo de documento: artigo
Estado:Versão publicada
Data de publicação:2015
País:Argentina
Recursos:Universidad Nacional de La Plata
Repositório:SEDICI (UNLP)
Idioma:inglês
OAI Identifier:oai:sedici.unlp.edu.ar:10915/133161
Acesso em linha:http://sedici.unlp.edu.ar/handle/10915/133161
Access Level:Acceso aberto
Palavra-chave:Química
Electrochemical Characterization
Hydrothermal Synthesis
Mwcnt
Ni/Mh Batteries
Nickel Electrode
Descrição
Resumo:The hydrothermal method was used to synthesize multi-walled carbon nanotube/nickel hydroxide composites (MWCNT/Ni(OH)<sub>2</sub>). The structure and morphology of the prepared materials were characterized by X-ray diffraction and transmission electron microscopy. The electrochemical performance of cathodes prepared with multi-walled carbon nanotubes (MWCNT) loaded into the β-nickel hydroxide materials was investigated employing cyclic voltammetry, galvanostatic charge/discharge and electrochemical impedance spectroscopic measurements. It is shown that the cathode active material utilization increases for MWCNT/Ni(OH)<sub>2</sub> obtained after 24 h of hydrothermal synthesis. These composites exhibit a fairly good electrochemical performance as cathode materials. Based on the results, this fact could be associated with the formation of a continuous conductive network structure in the hydroxide matrix. The analyses of impedance data, according to a physicochemical model, allow the improvement of a better understanding of the main structural and physicochemical parameters that control the electrochemical performance of these systems.