Extension of a classic theory of the low frequency dielectric dispersion of colloidal suspensions to the high frequency domain

The classic Shilov-Dukhin theory of the low frequency dielectric dispersion of colloidal suspensions in binary electrolyte solutions [Shilov, V. N.; Dukhin, S. S., Colloid J. 1970, 32, 245.; Dukhin, S. S.; Shilov, V. N. Dielectric Phenomena and the Double Layer in Disperse Systems and Polyelectrolyt...

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Detalhes bibliográficos
Autor: Grosse, Constantino
Tipo de documento: artigo
Estado:Versão publicada
Data de publicação:2010
País:Argentina
Recursos:Consejo Nacional de Investigaciones Científicas y Técnicas
Repositório:CONICET Digital (CONICET)
Idioma:inglês
OAI Identifier:oai:ri.conicet.gov.ar:11336/73568
Acesso em linha:http://hdl.handle.net/11336/73568
Access Level:Acceso aberto
Palavra-chave:Low Frequency Dielectric Dispersion
Maxwell-Wagner Dispersion
Broad Frequency Range
Wide Frequency Range
https://purl.org/becyt/ford/1.3
https://purl.org/becyt/ford/1
Descrição
Resumo:The classic Shilov-Dukhin theory of the low frequency dielectric dispersion of colloidal suspensions in binary electrolyte solutions [Shilov, V. N.; Dukhin, S. S., Colloid J. 1970, 32, 245.; Dukhin, S. S.; Shilov, V. N. Dielectric Phenomena and the Double Layer in Disperse Systems and Polyelectrolytes; Wiley: New York, 1974] was developed for the frequency range corresponding to the concentration polarization phenomenon: up to a few megahertz. While a few extensions to a broad frequency range including the Maxwell-Wagner-OKonski dispersion exist, they all consist of modifications of the final results of the theory rather than modifications of its hypothesis, extending their validity to high frequencies. In this work we avoid this artificial process by providing a high frequency extension fully from within the theory.