Thermal effects on helium scattering from LiF(001) at grazing incidence

Grazing-incidence fast atom diffraction (GIFAD) is an exceptionally sensitive method for surface analysis, which can be applied not only at room temperature but also at higher temperatures. In this work we use the He-LiF(001) system as a benchmark to study the influence of temperature on GIFAD patte...

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Detalles Bibliográficos
Autores: Frisco, Leandro, Gravielle, Maria Silvia
Tipo de recurso: artículo
Estado:Versión publicada
Fecha de publicación:2020
País:Argentina
Institución:Consejo Nacional de Investigaciones Científicas y Técnicas
Repositorio:CONICET Digital (CONICET)
Idioma:inglés
OAI Identifier:oai:ri.conicet.gov.ar:11336/151940
Acceso en línea:http://hdl.handle.net/11336/151940
Access Level:acceso abierto
Palabra clave:SURFACE
GRAZING INCIDENCE FAST ATOM DIFFRACTION
TEMPERATURE
PHONON
https://purl.org/becyt/ford/1.3
https://purl.org/becyt/ford/1
Descripción
Sumario:Grazing-incidence fast atom diffraction (GIFAD) is an exceptionally sensitive method for surface analysis, which can be applied not only at room temperature but also at higher temperatures. In this work we use the He-LiF(001) system as a benchmark to study the influence of temperature on GIFAD patterns from insulator surfaces. Our theoretical description is based on the phonon-surface initial value representation (P0-SIVR) approximation, which is a semiquantum approach that includes the phonon contribution to the elastic scattering. Within the P0-SIVR approach the main features introduced by thermal lattice vibrations on the angular distributions of scattered projectiles are investigated as a function of the crystal temperature. We found that azimuthal and polar spectra are strongly affected by thermal fluctuations, which modify the relative intensities and the polar spread of the interference structures. These findings are relevant for the use of GIFAD in surface research. Moreover, the present results are contrasted with available experimental data at room temperature.