Conformer-selective Photodynamics of TrpH+−H2O

The photodynamics of protonated tryptophan and its mono hydrated complex TrpH+−H2O has been revisited. A combination of steady-state IR and UV cryogenic ion spectroscopies with picosecond pump-probe photodissociation experiments sheds new lights on the deactivation processes of TrpH+ and conformer-s...

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Bibliographic Details
Authors: Molina, Franco Leonardo, Dezalay, Jordan, Tabata, Jun-ichi, Soorkia, Satchin, Broquier, Michel, Hirata, Keisuke, Ishiuchi, Shun-Ichi, Fujii, Masaaki, Grégoire, Gilles
Format: article
Status:Published version
Publication Date:2023
Country:Argentina
Institution:Consejo Nacional de Investigaciones Científicas y Técnicas
Repository:CONICET Digital (CONICET)
Language:English
OAI Identifier:oai:ri.conicet.gov.ar:11336/226761
Online Access:http://hdl.handle.net/11336/226761
Access Level:Open access
Keyword:BIOMOLECULES
CRYOGENIC ION SPECTROSCOPY
HYDRATION
IR AND UV PHOTODISSOCIATION
PHOTOPHYSICS
https://purl.org/becyt/ford/1.4
https://purl.org/becyt/ford/1
Description
Summary:The photodynamics of protonated tryptophan and its mono hydrated complex TrpH+−H2O has been revisited. A combination of steady-state IR and UV cryogenic ion spectroscopies with picosecond pump-probe photodissociation experiments sheds new lights on the deactivation processes of TrpH+ and conformer-selected TrpH+−H2O complex, supported by quantum chemistry calculations at the DFT and coupled-cluster levels for the ground and excited states, respectively. TrpH+ excited at the band origin exhibits a transient of less than 100 ps, assigned to the lifetime of the excited state proton transfer (ESPT) structure. The two experimentally observed conformers of TrpH+−H2O have been assigned. A striking result arises from the conformer-selective photodynamics of TrpH+−H2O, in which a single water molecule inserted in between the ammonium and the indole ring hinders the barrierless ESPT reaction responsible for the ultra-fast deactivation process observed in the other conformer and in bare TrpH+.