Novel bifunctional mesoporous catalysts based on Preyssler heteropolyacids for green pyrrole derivative synthesis

In this paper, we report the synthesis of Preyssler heteropolyacids supported on mesoporous alumina in order to obtain materials with acid–base properties. A series of pyrrole derivatives were synthesized using a suitable procedure under solvent-free conditions. Using the alumina-supported material,...

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Detalles Bibliográficos
Autores: Portilla Zúñiga, Omar Miguel, Sathicq, Ángel Gabriel, Martínez, José, Rojas, Hugo Santos, De Gerónimo, Eduardo, Luque, Rafael, Romanelli, Gustavo Pablo
Tipo de recurso: artículo
Estado:Versión publicada
Fecha de publicación:2018
País:Argentina
Institución:Universidad Nacional de La Plata
Repositorio:SEDICI (UNLP)
Idioma:inglés
OAI Identifier:oai:sedici.unlp.edu.ar:10915/97749
Acceso en línea:http://sedici.unlp.edu.ar/handle/10915/97749
Access Level:acceso abierto
Palabra clave:Química
Catalox SBA-90
Catalyst
Green chemistry
Preyssler heteropolyacids
Pyrroles
Descripción
Sumario:In this paper, we report the synthesis of Preyssler heteropolyacids supported on mesoporous alumina in order to obtain materials with acid–base properties. A series of pyrrole derivatives were synthesized using a suitable procedure under solvent-free conditions. Using the alumina-supported material, more complex pyrrole derivatives can be obtained through a tandem one-pot process that involves the formation of 2-amino-3-cyano 4-H-chromenes by a multicomponent reaction and their subsequent conversion to pyrrole using a Paal–Knorr reaction.