Stereochemical dependence of NMR geminal spin-spin coupling constants

In this work it was sought to explore the versatility of germinal spin–spin coupling constants, ²JxySSCCs, as probes for stereochemical studies. A set of compounds, where their experimental ²JxySSCCs through the X–C–Y molecular fragment are predicted to be sensitive to hyperconjugative interactions...

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Detalles Bibliográficos
Autores: Contreras, Ruben Horacio, Provasi, Patricio Federico, Dos Santos, Francisco P., Tormena, Claudio F.
Tipo de recurso: artículo
Estado:Versión publicada
Fecha de publicación:2008
País:Argentina
Institución:Consejo Nacional de Investigaciones Científicas y Técnicas
Repositorio:CONICET Digital (CONICET)
Idioma:inglés
OAI Identifier:oai:ri.conicet.gov.ar:11336/24680
Acceso en línea:http://hdl.handle.net/11336/24680
Access Level:acceso abierto
Palabra clave:Geminal Couplings
Nmr
Fermi Contact
Stereochemistry
Geminal Spin–Spin Coupling Constants
Stereochemical Analysis
https://purl.org/becyt/ford/1.3
https://purl.org/becyt/ford/1
Descripción
Sumario:In this work it was sought to explore the versatility of germinal spin–spin coupling constants, ²JxySSCCs, as probes for stereochemical studies. A set of compounds, where their experimental ²JxySSCCs through the X–C–Y molecular fragment are predicted to be sensitive to hyperconjugative interactions involving either bonding or antibonding orbitals containing the C carbon atom (‘coupling pathway’), were analyzed. SSCC calculations were performed for some selected examples using the second order polarization propagator approximation (SOPPA) method or within the DFT-B3LYP framework. Hyperconjugative interactions were calculated within the Natural Bond Orbital (NBO) approach. Results are condensed in two qualitative rules: Rule Iм—hyperconjugative interactions transferring charge into the coupling pathway yield a positive increase to the Fermi contact (FC), contribution to ²Kxy reduced spin–spin coupling constants (RSSCC), and Rule IIм—hyperconjugative interactions transferring charge from the coupling pathway yield a negative increase to the FC contribution to ²Kxy RSSCC.