Voltamperometric discrimination of urea and melamine adulterated skimmed milk powder

Nitrogen compounds like urea and melamine are known to be commonly used for milk adulteration resulting in undesired intoxication; a well-known example is the Chinese episode occurred in 2008. The development of a rapid, reliable and economic test is of relevance in order to improve adulterated milk...

ver descrição completa

Detalhes bibliográficos
Autores: Hilding-Ohlsson, A., Fauerbach, J.A., Sacco, N.J., Bonetto, M.C., Cortón, E.
Formato: artículo
Estado:Versión publicada
Fecha de publicación:2012
País:Argentina
Recursos:Universidad Nacional de Buenos Aires. Facultad de Ciencias Exactas y Naturales
Repositorio:Biblioteca Digital (UBA-FCEN)
Idioma:inglés
OAI Identifier:paperaa:paper_14248220_v12_n9_p12220_HildingOhlsson
Acesso em linha:http://hdl.handle.net/20.500.12110/paper_14248220_v12_n9_p12220_HildingOhlsson
Access Level:acceso abierto
Palavra-chave:F-PCA
KNN
Milk adulteration
Rapid screening methods
Voltammetry
Functional principal component analysis
Milk adulterations
Rapid screening
Screening methods
Significant differences
Voltammetric data
Cyclic voltammetry
Metabolism
Principal component analysis
Urea
melamine
triazine derivative
urea
animal
article
chemistry
dairy product
f-PCA
food contamination
methodology
milk
milk adulteration
potentiometry
powder
principal component analysis
rapid screening methods
voltammetry
Animals
Dairy Products
Food Contamination
Milk
Powders
Principal Component Analysis
Triazines
Descrição
Resumo:Nitrogen compounds like urea and melamine are known to be commonly used for milk adulteration resulting in undesired intoxication; a well-known example is the Chinese episode occurred in 2008. The development of a rapid, reliable and economic test is of relevance in order to improve adulterated milk identification. Cyclic voltammetry studies using an Au working electrode were performed on adulterated and non-adulterated milk samples from different independent manufacturers. Voltammetric data and their first derivative were subjected to functional principal component analysis (f-PCA) and correctly classified by the KNN classifier. The adulterated and non-adulterated milk samples showed significant differences. Best results of prediction were obtained with first derivative data. Detection limits in milk samples adulterated with 1% of its total nitrogen derived from melamine or urea were as low as 85.0 mg·L-1 and 121.4 mg·L-1, respectively. We present this method as a fast and robust screening method for milk adulteration analysis and prevention of food intoxication. © 2012 by the authors; licensee MDPI, Basel, Switzerland.