GC/MS Analyses of Thiosemicarbazones Synthesized from Acetophenones: Thermal Decay and Mass Spectra Features

The mass spectral fragmentation of thiosemicarbazones synthesized from acetophenones has been studied by CG/MS. These carbonyl compounds exhibit chromatographic peaks which are not observed in aliphatic analogues or those synthesized from aldehydes. The analysis of the corresponding spectra has allo...

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Detalles Bibliográficos
Autores: Gastaca, Belén, Galletti, Gastón Hernán, Sánchez, Hernán Rubén, Pis Diez, Reinaldo, Schiavoni, María de las Mercedes, Furlong, Jorge Javier Pedro
Tipo de recurso: artículo
Estado:Versión publicada
Fecha de publicación:2015
País:Argentina
Institución:Universidad Nacional de La Plata
Repositorio:SEDICI (UNLP)
Idioma:inglés
OAI Identifier:oai:sedici.unlp.edu.ar:10915/119281
Acceso en línea:http://sedici.unlp.edu.ar/handle/10915/119281
Access Level:acceso abierto
Palabra clave:Química
Thiosemicarbazones
Mass Spectrometry Analyses
Dimerization of Thiosemicarbazones
Descripción
Sumario:The mass spectral fragmentation of thiosemicarbazones synthesized from acetophenones has been studied by CG/MS. These carbonyl compounds exhibit chromatographic peaks which are not observed in aliphatic analogues or those synthesized from aldehydes. The analysis of the corresponding spectra has allowed structural assignment to the dimerization of gas phase neutral fragments. Theoretical calculations (DFT level) also provide evidence to support the experimental observations.