Covalent bond orders revisited: The open-shell case

This article states the concept of covalent bond order for open-shell systems from the invariance properties of the first- and second-order reduced density matrices for all the components of a multiplet state. A general bond order definition is formulated in the framework of the electronic populatio...

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Detalhes bibliográficos
Autores: Alcoba, Diego Ricardo, Bochicchio, Roberto Carlos, Blainq, Luis, Torres, Alicia Ines
Tipo de documento: artigo
Estado:Versão publicada
Data de publicação:2008
País:Argentina
Recursos:Consejo Nacional de Investigaciones Científicas y Técnicas
Repositório:CONICET Digital (CONICET)
Idioma:inglês
OAI Identifier:oai:ri.conicet.gov.ar:11336/64757
Acesso em linha:http://hdl.handle.net/11336/64757
Access Level:Acceso aberto
Palavra-chave:Reduced Density Materices
Covalent Bond Orders
Spin Density
https://purl.org/becyt/ford/1.3
https://purl.org/becyt/ford/1
Descrição
Resumo:This article states the concept of covalent bond order for open-shell systems from the invariance properties of the first- and second-order reduced density matrices for all the components of a multiplet state. A general bond order definition is formulated in the framework of the electronic population analyses in the Hilbert space of atomic orbitals. © the Owner Societies.