Gadolinium(III) and europium(III) L-glutamates: Synthesis and characterization

Two lanthanide(III) complexes with L-glutamate ligands [{Ln2(L-Glu)2(H2O)8}.4(ClO4).2.5H2O]n (Ln = Gd (1), Eu (2)) have been prepared and characterized by single-crystal X-ray diffraction. The compounds are isomorphous with infinite cationic 2D layers stacked together by secondary bonds. The buildin...

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Detalhes bibliográficos
Autores: Barja, Beatriz Carmen, Baggio, Ricardo, Calvo, Rafael, Garland, María, Perec, Mireille, Rizzi, Alberto Claudio
Formato: artículo
Estado:Versión publicada
Fecha de publicación:2006
País:Argentina
Recursos:Consejo Nacional de Investigaciones Científicas y Técnicas
Repositorio:CONICET Digital (CONICET)
Idioma:inglés
OAI Identifier:oai:ri.conicet.gov.ar:11336/26502
Acesso em linha:http://hdl.handle.net/11336/26502
Access Level:acceso abierto
Palavra-chave:Epr
Glutamates
Gadolinium And Europium
https://purl.org/becyt/ford/1.4
https://purl.org/becyt/ford/1
Descrição
Resumo:Two lanthanide(III) complexes with L-glutamate ligands [{Ln2(L-Glu)2(H2O)8}.4(ClO4).2.5H2O]n (Ln = Gd (1), Eu (2)) have been prepared and characterized by single-crystal X-ray diffraction. The compounds are isomorphous with infinite cationic 2D layers stacked together by secondary bonds. The building blocks are slightly different non-centrosymmetric dinuclear units placed in alternating layers, the resulting structures thus containing four non-equivalent Ln metal sites. The dinuclear units contain a fourfold bridge, two in the eta1:eta1:mi2 and two in the eta2:eta1:mi2 modes, from two alfa- and two gamma-carboxylates of four different L-Glu residues, respectively.