The role of multiple ionization of H2O in heavy ion collisions

Collisional ionization processes involving H2O molecules and C6+, O8+, Si13+ ions are studied by means of the classical trajectory Monte Carlo method using molecular orbital calculations to define the ionization stages of the water molecule. Net total and single-differential cross sectionsin energy...

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Detalles Bibliográficos
Autores: Bachi, Nicolás, Otranto, Sebastián, Otero, Guadalupe Sol, Olson, Ronald E.
Tipo de recurso: artículo
Estado:Versión publicada
Fecha de publicación:2019
País:Argentina
Institución:Consejo Nacional de Investigaciones Científicas y Técnicas
Repositorio:CONICET Digital (CONICET)
Idioma:inglés
OAI Identifier:oai:ri.conicet.gov.ar:11336/119270
Acceso en línea:http://hdl.handle.net/11336/119270
Access Level:acceso abierto
Palabra clave:CROSS SECTIONS
HEAVY ION COLLISIONS
RADIOTHERAPY
SINGLE AND MULTIPLE IONIZATION
WATER
https://purl.org/becyt/ford/1.3
https://purl.org/becyt/ford/1
Descripción
Sumario:Collisional ionization processes involving H2O molecules and C6+, O8+, Si13+ ions are studied by means of the classical trajectory Monte Carlo method using molecular orbital calculations to define the ionization stages of the water molecule. Net total and single-differential cross sectionsin energy and angle are obtained by using a newly developed model that goes beyond the commonly applied oneactive electron approximation. This model allows us to access the fraction of electron emission arising from single and multiple electron ionization. Calculated cross sections are contrasted and benchmarked against available experimental data at impact energies in the MeV/u range. The present results highlight the important role of multiple ionization in the emission of electrons where we find the majority of electrons emitted with energies greater than ~50eV arise from multiple ionization collisions.