Thermal characterization of novel p-nitrobenzylacrylate-diisopropyl fumarate copolymer synthesized under microwave energy

Copolymers of p-nitrobenzyl acrylate and diisopropyl fumarate with different feed ratios were synthesized under microwave and thermal heating conditions, and then characterized by IR, 1H-, and 13C-NMR spectroscopy. Average molecular weights were analyzed by size exclusion chromatography (SEC). Monom...

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Detalles Bibliográficos
Autores: Oberti, Tamara Gisela, Alessandrini, José Luis, Cortizo, Maria Susana
Tipo de recurso: artículo
Estado:Versión publicada
Fecha de publicación:2012
País:Argentina
Institución:Consejo Nacional de Investigaciones Científicas y Técnicas
Repositorio:CONICET Digital (CONICET)
Idioma:inglés
OAI Identifier:oai:ri.conicet.gov.ar:11336/82166
Acceso en línea:http://hdl.handle.net/11336/82166
Access Level:acceso abierto
Palabra clave:Glass Transition Temperature
Microwave Polymerization
P-Nitrobenzyl Acrylate
Thermal Degradation
Thermogravimetry Analysis
https://purl.org/becyt/ford/1.4
https://purl.org/becyt/ford/1
Descripción
Sumario:Copolymers of p-nitrobenzyl acrylate and diisopropyl fumarate with different feed ratios were synthesized under microwave and thermal heating conditions, and then characterized by IR, 1H-, and 13C-NMR spectroscopy. Average molecular weights were analyzed by size exclusion chromatography (SEC). Monomer reactivity ratios were obtained from an extended Kelen-Tüdös method. Differential scanning calorimetry and thermogravimetry were used to evaluate the thermal behavior of all copolymers synthesized under microwave energy. Based on the products analyzed by SEC and gas chromatography-mass spectrometry, a possible mechanism of degradation is postulated.