Experimental study of CO2 convective dissolution: The effect of color indicators

Color indicators are often used for visualization purposes in experimental studies of CO2 convective dissolution in aqueous solutions. We analyze and compare here experimentally the hydrodynamic fingering pattern induced by CO2 dissolution in aqueous solutions of various color indicators. Characteri...

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Detalhes bibliográficos
Autores: Thomas Carazo, María del Carmen, Lemaigre, L., Zalts, Anita, D'onofrio, Alejandro Gustavo, De Wit, A.
Formato: artículo
Estado:Versión publicada
Fecha de publicación:2015
País:Argentina
Recursos:Consejo Nacional de Investigaciones Científicas y Técnicas
Repositorio:CONICET Digital (CONICET)
Idioma:inglés
OAI Identifier:oai:ri.conicet.gov.ar:11336/38555
Acesso em linha:http://hdl.handle.net/11336/38555
Access Level:acceso abierto
Palavra-chave:Co2 Sequestration
Color Indicator
Convective Dissolution
Fingering
Reactive Dissolution
https://purl.org/becyt/ford/1.5
https://purl.org/becyt/ford/1
Descrição
Resumo:Color indicators are often used for visualization purposes in experimental studies of CO2 convective dissolution in aqueous solutions. We analyze and compare here experimentally the hydrodynamic fingering pattern induced by CO2 dissolution in aqueous solutions of various color indicators. Characteristics of the convective patterns are measured as a function of time to study whether the choice of the color indicator or its concentration has an influence on the dynamics. We also compare the visualization of the fingering instability with a color indicator to the pattern observed with a Schlieren technique tracking changes in index of refraction. We find that color indicators are able only to track pH isocurves and do not always allow to capture the full extent of the fingers. We conclude that color indicators should be used with caution in experimental works devoted to quantify properties of CO2 convective dissolution.