Critical aspects in the production of periodically ordered mesoporous titania thin films
Periodically ordered mesoporous titania thin films (MTTF) present a high surface area, controlled porosity in the 2-20 nm pore diameter range and an amorphous or crystalline inorganic framework. These materials are nowadays routinely prepared by combining soft chemistry and supramolecular templating...
| Autores: | , , , , |
|---|---|
| Tipo de recurso: | artículo |
| Estado: | Versión publicada |
| Fecha de publicación: | 2012 |
| País: | Argentina |
| Institución: | Consejo Nacional de Investigaciones Científicas y Técnicas |
| Repositorio: | CONICET Digital (CONICET) |
| Idioma: | inglés |
| OAI Identifier: | oai:ri.conicet.gov.ar:11336/194948 |
| Acceso en línea: | http://hdl.handle.net/11336/194948 |
| Access Level: | acceso abierto |
| Palabra clave: | Mesoporous Titanium dioxide Nanocrystalline thin films Photocatalysis Solar Cells https://purl.org/becyt/ford/2.10 https://purl.org/becyt/ford/2 |
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Critical aspects in the production of periodically ordered mesoporous titania thin filmsSoler Illia, Galo Juan de Avila ArturoAngelome, Paula CeciliaFuertes, María CeciliaGrosso, DavidBoissiere, CedricMesoporous Titanium dioxideNanocrystalline thin filmsPhotocatalysisSolar Cellshttps://purl.org/becyt/ford/2.10https://purl.org/becyt/ford/2Periodically ordered mesoporous titania thin films (MTTF) present a high surface area, controlled porosity in the 2-20 nm pore diameter range and an amorphous or crystalline inorganic framework. These materials are nowadays routinely prepared by combining soft chemistry and supramolecular templating. Photocatalytic transparent coatings and titania-based solar cells are the immediate promising applications. However, a wealth of new prospective uses have emerged on the horizon, such as advanced catalysts, perm-selective membranes, optical materials based on plasmonics and photonics, metamaterials, biomaterials or new magnetic nanocomposites. Current and novel applications rely on the ultimate control of the materials features such as pore size and geometry, surface functionality and wall structure. Even if a certain control of these characteristics has been provided by the methods reported so far, the needs for the next generation of MTTF require a deeper insight in the physical and chemical processes taking place in their preparation and processing. This article presents a critical discussion of these aspects. This discussion is essential to evolve from know-how to sound knowledge, aiming at a rational materials design of these fascinating systems.Fil: Soler Illia, Galo Juan de Avila Arturo. Departamento Fundamentos y Aplicaciones de la Quimica ; Gerencia de Quimica (cac) ; Comision Nacional de Energia Atomica; . Consejo Nacional de Investigaciones Científicas y Técnicas; ArgentinaFil: Angelome, Paula Cecilia. Departamento Fundamentos y Aplicaciones de la Quimica ; Gerencia de Quimica (cac) ; Comision Nacional de Energia Atomica; . Consejo Nacional de Investigaciones Científicas y Técnicas; ArgentinaFil: Fuertes, María Cecilia. Departamento Fundamentos y Aplicaciones de la Quimica ; Gerencia de Quimica (cac) ; Comision Nacional de Energia Atomica; . Consejo Nacional de Investigaciones Científicas y Técnicas; ArgentinaFil: Grosso, David. Universite de Paris VI; Francia. Centre National de la Recherche Scientifique; FranciaFil: Boissiere, Cedric. Universite de Paris VI; Francia. Centre National de la Recherche Scientifique; FranciaRoyal Society of Chemistry2012-02-10info:eu-repo/semantics/articleinfo:eu-repo/semantics/publishedVersionhttp://purl.org/coar/resource_type/c_6501info:ar-repo/semantics/articuloapplication/pdfapplication/pdfapplication/pdfapplication/pdfhttp://hdl.handle.net/11336/194948Soler Illia, Galo Juan de Avila Arturo; Angelome, Paula Cecilia; Fuertes, María Cecilia; Grosso, David; Boissiere, Cedric; Critical aspects in the production of periodically ordered mesoporous titania thin films; Royal Society of Chemistry; Nanoscale; 4; 8; 10-2-2012; 2549-25662040-33642040-3372CONICET DigitalCONICETenginfo:eu-repo/semantics/altIdentifier/url/https://pubs.rsc.org/en/content/articlelanding/2012/nr/c2nr11817cinfo:eu-repo/semantics/altIdentifier/doi/10.1039/C2NR11817Cinfo:eu-repo/semantics/openAccesshttps://creativecommons.org/licenses/by-nc-sa/2.5/ar/reponame:CONICET Digital (CONICET)instname:Consejo Nacional de Investigaciones Científicas y Técnicas2024-05-08T13:38:43Zoai:ri.conicet.gov.ar:11336/194948instacron:CONICETInstitucionalhttp://ri.conicet.gov.ar/Organismo científico-tecnológicoNo correspondehttp://ri.conicet.gov.ar/oai/requestdasensio@conicet.gov.ar; lcarlino@conicet.gov.arArgentinaNo correspondeNo correspondeNo correspondeopendoar:34982024-05-08 13:38:43.582CONICET Digital (CONICET) - Consejo Nacional de Investigaciones Científicas y Técnicasfalse |
| dc.title.none.fl_str_mv |
Critical aspects in the production of periodically ordered mesoporous titania thin films |
| title |
Critical aspects in the production of periodically ordered mesoporous titania thin films |
| spellingShingle |
Critical aspects in the production of periodically ordered mesoporous titania thin films Soler Illia, Galo Juan de Avila Arturo Mesoporous Titanium dioxide Nanocrystalline thin films Photocatalysis Solar Cells https://purl.org/becyt/ford/2.10 https://purl.org/becyt/ford/2 |
| title_short |
Critical aspects in the production of periodically ordered mesoporous titania thin films |
| title_full |
Critical aspects in the production of periodically ordered mesoporous titania thin films |
| title_fullStr |
Critical aspects in the production of periodically ordered mesoporous titania thin films |
| title_full_unstemmed |
Critical aspects in the production of periodically ordered mesoporous titania thin films |
| title_sort |
Critical aspects in the production of periodically ordered mesoporous titania thin films |
| dc.creator.none.fl_str_mv |
Soler Illia, Galo Juan de Avila Arturo Angelome, Paula Cecilia Fuertes, María Cecilia Grosso, David Boissiere, Cedric |
| author |
Soler Illia, Galo Juan de Avila Arturo |
| author_facet |
Soler Illia, Galo Juan de Avila Arturo Angelome, Paula Cecilia Fuertes, María Cecilia Grosso, David Boissiere, Cedric |
| author_role |
author |
| author2 |
Angelome, Paula Cecilia Fuertes, María Cecilia Grosso, David Boissiere, Cedric |
| author2_role |
author author author author |
| dc.subject.none.fl_str_mv |
Mesoporous Titanium dioxide Nanocrystalline thin films Photocatalysis Solar Cells https://purl.org/becyt/ford/2.10 https://purl.org/becyt/ford/2 |
| topic |
Mesoporous Titanium dioxide Nanocrystalline thin films Photocatalysis Solar Cells https://purl.org/becyt/ford/2.10 https://purl.org/becyt/ford/2 |
| description |
Periodically ordered mesoporous titania thin films (MTTF) present a high surface area, controlled porosity in the 2-20 nm pore diameter range and an amorphous or crystalline inorganic framework. These materials are nowadays routinely prepared by combining soft chemistry and supramolecular templating. Photocatalytic transparent coatings and titania-based solar cells are the immediate promising applications. However, a wealth of new prospective uses have emerged on the horizon, such as advanced catalysts, perm-selective membranes, optical materials based on plasmonics and photonics, metamaterials, biomaterials or new magnetic nanocomposites. Current and novel applications rely on the ultimate control of the materials features such as pore size and geometry, surface functionality and wall structure. Even if a certain control of these characteristics has been provided by the methods reported so far, the needs for the next generation of MTTF require a deeper insight in the physical and chemical processes taking place in their preparation and processing. This article presents a critical discussion of these aspects. This discussion is essential to evolve from know-how to sound knowledge, aiming at a rational materials design of these fascinating systems. |
| publishDate |
2012 |
| dc.date.none.fl_str_mv |
2012-02-10 |
| dc.type.none.fl_str_mv |
info:eu-repo/semantics/article info:eu-repo/semantics/publishedVersion http://purl.org/coar/resource_type/c_6501 info:ar-repo/semantics/articulo |
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article |
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publishedVersion |
| dc.identifier.none.fl_str_mv |
http://hdl.handle.net/11336/194948 Soler Illia, Galo Juan de Avila Arturo; Angelome, Paula Cecilia; Fuertes, María Cecilia; Grosso, David; Boissiere, Cedric; Critical aspects in the production of periodically ordered mesoporous titania thin films; Royal Society of Chemistry; Nanoscale; 4; 8; 10-2-2012; 2549-2566 2040-3364 2040-3372 CONICET Digital CONICET |
| url |
http://hdl.handle.net/11336/194948 |
| identifier_str_mv |
Soler Illia, Galo Juan de Avila Arturo; Angelome, Paula Cecilia; Fuertes, María Cecilia; Grosso, David; Boissiere, Cedric; Critical aspects in the production of periodically ordered mesoporous titania thin films; Royal Society of Chemistry; Nanoscale; 4; 8; 10-2-2012; 2549-2566 2040-3364 2040-3372 CONICET Digital CONICET |
| dc.language.none.fl_str_mv |
eng |
| language |
eng |
| dc.relation.none.fl_str_mv |
info:eu-repo/semantics/altIdentifier/url/https://pubs.rsc.org/en/content/articlelanding/2012/nr/c2nr11817c info:eu-repo/semantics/altIdentifier/doi/10.1039/C2NR11817C |
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info:eu-repo/semantics/openAccess https://creativecommons.org/licenses/by-nc-sa/2.5/ar/ |
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openAccess |
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https://creativecommons.org/licenses/by-nc-sa/2.5/ar/ |
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application/pdf application/pdf application/pdf application/pdf |
| dc.publisher.none.fl_str_mv |
Royal Society of Chemistry |
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Royal Society of Chemistry |
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reponame:CONICET Digital (CONICET) instname:Consejo Nacional de Investigaciones Científicas y Técnicas |
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Consejo Nacional de Investigaciones Científicas y Técnicas |
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CONICET Digital (CONICET) |
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CONICET Digital (CONICET) |
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CONICET Digital (CONICET) - Consejo Nacional de Investigaciones Científicas y Técnicas |
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dasensio@conicet.gov.ar; lcarlino@conicet.gov.ar |
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1799194897141465088 |
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15,812429 |